Prof. Dr. Daniel Loss

Molecular nanomagnets show clear signatures of coherent behavior and have a wide variety of effective low-energy spin Hamiltonians suitable for encoding qubits and implementing spin-based quantum information processing. At the nanoscale, the preferred mechanism for control of quantum systems is through application of electric fields, which are strong, can be locally applied, and rapidly switched. In this work, we provide the theoretical tools for the search for single molecule magnets suitable for electric control. By group-theoretical symmetry analysis we find that the spin-electric coupling in triangular molecules is governed by the modification of the exchange interaction, and is possible even in the absence of spin-orbit coupling. In pentagonal molecules the spin-electric coupling can exist only in the presence of spin-orbit interaction. This kind of coupling is allowed for both s = 1/2 and s = 3/2 spins at the magnetic centers. Within the Hubbard model, we find a relation between the spin-electric coupling and the properties of the chemical bonds in a molecule, suggesting that the best candidates for strong spin-electric coupling are molecules with nearly degenerate bond orbitals. We also investigate the possible experimental signatures of spin-electric coupling in nuclear magnetic resonance and electron spin resonance spectroscopy, as well as in the thermodynamic measurements of magnetization, electric polarization, and specific heat of the molecules.

We evaluate free-induction decay for the transverse components of a localized electron spin coupled to a bath of nuclear spins via the Fermi contact hyperfine interaction. Our perturbative treatment is valid for special (narrowed) bath initial conditions and when the Zeeman energy of the electron $b$ exceeds the total hyperfine coupling constant $A$: $b>A$. Using one unified and systematic method, we recover previous results reported at short and long times using different techniques. We find a new and unexpected modulation of the free-induction-decay envelope, which is present even for a purely isotropic hyperfine interaction without spin echoes and for a single nuclear species. We give sub-leading corrections to the decoherence rate, and show that, in general, the decoherence rate has a non-monotonic dependence on electron Zeeman splitting, leading to a pronounced maximum. These results illustrate the limitations of methods that make use of leading-order effective Hamiltonians and re-exponentiation of short-time expansions for a strongly-interacting system with non-Markovian (history-dependent) dynamics.

We propose a one-step scheme to generate GHZ states for superconducting flux qubits or charge qubits in a circuit QED setup. The GHZ state can be produced within the coherence time of the multi-qubit system. Our scheme is independent of the initial state of the transmission line resonator and works in the presence of higher harmonic modes. Our analysis also shows that the scheme is robust to various operation errors and environmental noise.

We study interfaces between graphene and graphane. If the interface is oriented along a zigzag direction, edge states are found which exhibit a strong amplification of effects related to the spin-orbit interaction. The enhanced spin splitting of the edge states allows a conversion between valley polarization and spin polarization at temperatures near one Kelvin. We show that these edge states give rise to quantum spin and/or valley Hall effects.

We calculate the electrically induced spin accumulation in diffusive systems due to both Rashba (with strength $\alpha)$ and Dresselhaus (with strength $\beta)$ spin-orbit interaction. Using a diffusion equation approach we find that magnetoelectric effects disappear and that there is thus no spin accumulation when both interactions have the same strength, $\alpha=\pm \beta$. In thermodynamically large systems, the finite spin accumulation predicted by Chaplik, Entin and Magarill, [Physica E 13, 744 (2002)] and by Trushin and Schliemann [Phys. Rev. B 75, 155323 (2007)] is recovered an infinitesimally small distance away from the singular point $\alpha=\pm \beta$. We show however that the singularity is broadened and that the suppression of spin accumulation becomes physically relevant (i) in finite-sized systems of size $L$, (ii) in the presence of a cubic Dresselhaus interaction of strength $\gamma$, or (iii) for finite frequency measurements. We obtain the parametric range over which the magnetoelectric effect is suppressed in these three instances as (i) $|\alpha|-|\beta| \lesssim 1/mL$, (ii)$|\alpha|-|\beta| \lesssim \gamma p_{\rm F}^2$, and (iii) $|\alpha|-|\beta| \lesssiM \sqrt{\omega/m p_{\rm F}\ell}$ with $\ell$ the elastic mean free path and $p_{\rm F}$ the Fermi momentum. We attribute the absence of spin accumulation close to $\alpha=\pm \beta$ to the underlying U (1) symmetry. We illustrate and confirm our predictions numerically.

We derive boundary conditions for the electrically induced spin accumulation in a finite 2D semiconductor channel. While for DC electric fields these boundary conditions select spatially constant spin profiles equivalent to a vanishing spin-Hall effect, we show that an in-plane ac electric field results in a non-zero ac spin-Hall effect, i.e., it generates a spatially non-uniform out-of-plane polarization even for linear intrinsic spin-orbit interactions. Analyzing different geometries in [001] and [110]-grown quantum wells, we find that although this out-of-plane polarization is typically confined to within a few spin-orbit lengths from the channel edges, it is also possible to generate spatially oscillating spin profiles which extend over the whole channel. The latter is due to the excitation of a driven spin-helix mode in the transverse direction of the channel. We show that while finite frequencies suppress this mode, it can be amplified by a magnetic field tuned to resonance with the frequency of the electric field. In this case, finite size effects at equal strengths of Rashba- and Dresselhaus SOI lead to an enhancement of the magnitude of this helix mode. We comment on the relation between spin currents and boundary conditions. http://prb.aps.org/kaleidoscope

The ability to store information is of fundamental importance to any computer, be it classical or quantum. Identifying systems for quantum memories which rely, analogously to classical memories, on passive error protection ('self-correction') is of greatest interest in quantum information science. While systems with topological ground states have been considered to be promising candidates, a large class of them was recently proven unstable against thermal fluctuations. Here, we propose new two-dimensional (2D) spin models unaffected by this result. Specifically, we introduce repulsive long-range interactions in the toric code and establish a memory lifetime polynomially increasing with the system size. This remarkable stability is shown to originate directly from the repulsive long-range nature of the interactions. We study the time dynamics of the quantum memory in terms of diffusing anyons and support all our analytical results with extensive numerical simulations. Our findings demonstrate that self-correcting quantum memories can exist in 2D at finite temperatures.

With the help of the spin-orbit interaction, we propose a scheme to perform holonomic single qubit gates on the electron spin confined to a quantum dot. The manipulation is done in the absence (or presence) of an applied magnetic field. By adiabatic changing the position of the confinement potential, one can rotate the spin state of the electron around the Bloch sphere in semiconductor heterostructures. The dynamics of the system is equivalent to employing an effective non-Abelian gauge potential whose structure depends on the type of the spin-orbit interaction. As an example, we find an analytic expression for the electron spin dynamics when the dot is moved around a circular path (with radius R) on the two dimensional electron gas (2DEG), and show that all single qubit gates can be realized by tuning the radius and orientation of the circular paths. Moreover, using the Heisenberg exchange interaction, we demonstrate how one can generate two-qubit gates by bringing two quantum dots near each other, yielding a scalable scheme to perform quantum computing on arbitrary N qubits. This proposal shows a way of realizing holonomic quantum computers in solid-state systems.

The interaction between localized magnetic moments and the electrons of a one-dimensional conductor can lead to an ordered phase in which the magnetic moments and the electrons are tightly bound to each other. We show here that this occurs when a lattice of nuclear spins is embedded in a Luttinger liquid. Experimentally available examples of such a system are single wall carbon nanotubes grown entirely from 13C and GaAs-based quantum wires. In these systems the hyperfine interaction between the nuclear spin and the conduction electron spin is very weak, yet it triggers a strong feedback reaction that results in an ordered phase consisting of a nuclear helimagnet that is inseparably bound to an electronic density wave combining charge and spin degrees of freedom. This effect can be interpreted as a strong renormalization of the nuclear Overhauser field and is a unique signature of Luttinger liquid physics. Through the feedback the order persists up into the millikelvin range. A particular signature is the reduction of the electric conductance by the universal factor 2.

We investigate the intrinsic spin Hall effect in two-dimensional electron gases in quantum wells with two subbands, where a new intersubband-induced spin-orbit coupling is operative. The bulk spin Hall conductivity $\sigma^z_xy$ is calculated in the ballistic limit within the standard Kubo formalism in the presence of a magnetic field $B$ and is found to remain finite in the B=0 limit, as long as only the lowest subband is occupied. Our calculated $\sigma^z_xy$ exhibits a non-monotonic behavior and can change its sign as the Fermi energy (the carrier areal density $n_2D$) is varied between the subband edges. We determine the magnitude of $\sigma^z_xy$ for realistic InSb quantum wells by performing a self-consistent calculation of the intersubband-induced spin-orbit coupling.

We discuss and review several thermodynamic criteria that have been introduced to characterize the thermal stability of a self-correcting quantum memory. We first examine the use of symmetry-breaking fields in analyzing the properties of self-correcting quantum memories in the thermodynamic limit: we show that the thermal expectation values of all logical operators vanish for any stabilizer and any subsystem code in any spatial dimension. On the positive side, we generalize the results in [R. Alicki et al., arXiv:0811.0033] to obtain a general upper bound on the relaxation rate of a quantum memory at nonzero temperature, assuming that the quantum memory interacts via a Markovian master equation with a thermal bath. This upper bound is applicable to quantum memories based on either stabilizer or subsystem codes.

We analyze Dicke model at zero temperature by matrix diagonalization to determine the entanglement in the ground state. In the infinite system limit the mean field approximation predicts a quantum phase transition from a non-interacting state to a Bose-Einstein condensate at a threshold coupling. We show that in a finite system the spin part of the ground state is a bipartite entangled state, which can be tested by probing two parts of the spin system separately, but only in a narrow regime around the threshold coupling. Around the resonance, the size of this regime is inversely proportional to the number of spins and shrinks down to zero for infinite systems. This spin entanglement is a non-perturbative effect and is also missed by the mean-field approximation.

Several topics on the implementation of spin qubits in quantum dots are reviewed. We first provide an introduction to the standard model of quantum computing and the basic criteria for its realization. Other alternative formulations such as measurement-based and adiabatic quantum computing are briefly discussed. We then focus on spin qubits in single and double GaAs electron quantum dots and review recent experimental achievements with respect to initialization, coherent manipulation and readout of the spin states. We extensively discuss the problem of decoherence in this system, with particular emphasis on its theoretical treatment and possible ways to overcome it.

We analytically calculate the nuclear-spin interactions of a single electron confined to a carbon nanotube or graphene quantum dot. While the conduction-band states in graphene are p-type, the accordant states in a carbon nanotube are sp-hybridized due to curvature. This leads to an interesting interplay between isotropic and anisotropic hyperfine interactions. By using only analytical methods, we are able to show how the interaction strength depends on important physical parameters, such as curvature and isotope abundances. We show that for the investigated carbon structures, the 13C hyperfine coupling strength is less than 1 mu-eV, and that the associated electron-spin decoherence time can be expected to be as long as several tens of microseconds, depending on the abundance of spin-carrying 13C nuclei. Furthermore, we find an unusual hyperfine-induced alignment of the 13C nuclear spins in nanotubes of any chirality.

The dream of building computers that work according to the rules of quantum mechanics has strongly driven research over the past decade in many fields of basic and applied sciences, including physics, chemistry, and computer science. About 10 years ago, it was shown mathematically that the direct use of quantum phenomena such as interference and entanglement could crucially speed up data searching and prime factorization for encryption. To turn quantum computers into reality, however, many issues in engineering and in basic physics need to be addressed.

We present two ready-to-use numerical algorithms to evaluate convex-roof extensions of arbitrary pure-state entanglement monotones. Their implementation leaves the user merely with the task of calculating derivatives of the respective pure-state measure. We provide numerical tests of the algorithms and demonstrate their good convergence properties. We further employ them in order to investigate the entanglement in particular few-spins systems at finite temperature. Namely, we consider ferromagnetic Heisenberg exchange-coupled spin-1/2 rings subject to an inhomogeneous in-plane field geometry obeying full rotational symmetry around the axis perpendicular to the ring through its center. We demonstrate that highly entangled states can be obtained in these systems at sufficiently low temperatures and by tuning the strength of a magnetic field configuration to an optimal value which is identified numerically.

Experiments in 13C nanotubes reveal surprisingly strong nuclear spin effects that, if properly harnessed, could provide a mechanism for manipulation and storage of quantum information.

We review recent studies on spin decoherence of electrons and holes in quasi-two-dimensional quantum dots, as well as electron-spin relaxation in nanowire quantum dots. The spins of confined electrons and holes are considered major candidates for the realization of quantum information storage and processing devices, provided that sufficently long coherence and relaxation times can be achieved. The results presented here indicate that this prerequisite might be realized in both electron and hole quantum dots, taking one large step towards quantum computation with spin qubits.

We present a semi-automated computer-assisted method to generate and calculate diagrams in the disorder averaging approach to disordered 2D conductors with intrinsic spin-orbit interaction (SOI). As an application, we calculate the effect of the SOI on the charge conductivity for disordered 2D systems and rings in the presence of Rashba and Dresselhaus SOI. In an infinite-size 2D system, anisotropic corrections to the conductivity tensor arise due to phase-coherence and the interplay of Rashba and Dresselhaus SOI. The effect is more pronounced in the quasi-onedimensional case, where the conductivity becomes anisotropic already in the presence of only one type of SOI. The anisotropy further increases if the time-reversal symmetry of the Hamiltonian is broken.

We investigate theoretically spin relaxation in heavy hole quantum dots in low external magnetic fields. We demonstrate that two-phonon processes and spin-orbit interaction are experimentally relevant and provide an explanation for the recently observed saturation of the spin relaxation rate in heavy hole quantum dots with vanishing magnetic fields. We propose further experiments to identify the relevant spin relaxation mechanisms in low magnetic fields.

Quantum measurements are conventionally thought of as irretrievably "collapsing" a wave function to the observed state. However, experiments with superconducting qubits show that the partial collapse resulting from a weak continuous measurement can be restored.

We study the coherent transport of heavy holes through a one-dimensional ring in the presence of spin-orbit coupling. Spin-orbit interaction of holes, cubic in the in-plane components of momentum, gives rise to an angular momentum dependent spin texture of the eigenstates and influences transport. We analyze the dependence of the resulting differential conductance of the ring on hole polarization of the leads and the signature of the textures in the Aharonov-Bohm oscillations when the ring is in a perpendicular magnetic field. We find that the polarization-resolved conductance reveals whether the dominant spin-orbit coupling is of Dresselhaus or Rashba type, and that the cubic spin-orbit coupling can be distinguished from the conventional linear coupling by observing the four-peak structure in the Aharonov-Bohm oscillations.

We study the time dynamics of a single boson coupled to a bath of two-level systems (spins 1/2) with different excitation energies, described by an inhomogeneous Dicke model. Solving the time-dependent Schroedinger equation exactly we find that at resonance the boson decays in time to an oscillatory state characterized by a single Rabi frequency. In the limit of small inhomogeneity, the decay is suppressed and exhibits a complex (mainly Gaussian-like) behavior, whereas the decay is complete and of exponential form in the opposite limit. For intermediate inhomogeneity, the boson decay is partial and governed by a combination of exponential and power laws.

We consider the effect of rescattering of pairs of quasiparticles in the Cooper channel resulting in the strong renormalization of second order corrections to the spin susceptibility in a two-dimensional electron system. We use the Fourier expansion of the scattering potential in the vicinity of the Fermi surface to find that each harmonic becomes renormalized independently. Since some of those harmonics are negative, the slope of the spin susceptibility is bound to be negative at small momenta, in contrast to the lowest order perturbation theory result, which predicts a positive slope. We present in detail an effective method to calculate diagrammatically corrections to the spin susceptibility to infinite order.

Theories of the spin Hall effect suggest that spin currents generated by electric fields accumulate spin polarization at the sample edges. Now an experiment has observed this conversion in real time.

The hyperfine interaction between the electron spin and the nuclear spins is one of the main sources of decoherence for spin qubits when the nuclear spins are disordered. An ordering of the latter largely suppresses this source of decoherence. Here we show that such an ordering can occur through a thermodynamic phase transition in two-dimensional (2D) Kondo-lattice type systems. We specifically focus on nuclear spins embedded in a 2D electron gas. The nuclear spins interact with each other through the RKKY interaction, which is carried by the electron gas. We show that a nuclear magnetic order at finite temperature relies on the anomalous behavior of the 2D static electron spin susceptibility due to electron-electron interactions. This provides a connection between low-dimensional magnetism and non-analyticities in interacting 2D electron systems. We discuss the conditions for nuclear magnetism, and show that the associated Curie temperature increases with the electron-electron interactions and may reach up into the millikelvin regime. The further reduction of dimensionality to one dimension is shortly discussed.

Nuclear spins embedded in correlated metals offer an ideal platform to investigate the effect of electron-electron interactions on magnetism of localized moments. Here we focus on a one-dimensional realization of such a system: Single wall carbon nanotubes grown entirely from the 13C isotope. With this isotope the nanotube forms a nuclear spin lattice which couples through the hyperfine interaction to a Luttinger liquid if the nanotube is in the metallic regime. Even though the hyperfine interaction is very weak, the system is driven into an ordered phase which combines electron and nuclear spin degrees of freedom. This phase persists up into the millikelvin regime and leads to a reduction of the nanotube conductance by a universal factor of 2, allowing for an experimental detection by standard transport measurements.

We study the spin stiffness of a one-dimensional quantum antiferromagnet in the whole range of system sizes L and temperatures T. We show that for integer and half-odd integer spin cases the stiffness differs fundamentally in its L and T dependences, and that in the latter case the stiffness exhibits a striking dependence on the parity of the number of sites. Integer spin chains are treated in terms of the nonlinear sigma model, while half-odd integer spin chains are discussed in a renormalization group approach leading to a Luttinger liquid with Aharonov-Bohm-type boundary conditions.

Recently, we have found an additional spin-orbit (SO) interaction in quantum wells with two subbands [Phys. Rev. Lett. 99, 076603 (2007)]. This new SO term is non-zero even in symmetric geometries, as it arises from the intersubband coupling between confined states of distinct parities, and its strength is comparable to that of the ordinary Rashba. Starting from the $8 \times 8$ Kane model, here we present a detailed derivation of this new SO Hamiltonian and the corresponding SO coupling. In addition, within the self-consistent Hartree approximation, we calculate the strength of this new SO coupling for realistic symmetric modulation-doped wells with two subbands. We consider gated structures with either a constant areal electron density or a constant chemical potential. In the parameter range studied, both models give similar results. By considering the effects of an external applied bias, which breaks the structural inversion symmetry of the wells, we also calculate the strength of the resulting induced Rashba couplings within each subband. Interestingly, we find that for double wells the Rashba couplings for the first and second subbands interchange signs abruptly across the zero bias, while the intersubband SO coupling exhibits a resonant behavior near this symmetric configuration. For completeness we also determine the strength of the Dresselhaus couplings and find them essentially constant as function of the applied bias.

We theoretically study the interaction of a heavy hole with nuclear spins in a quasi-two-dimensional III-V semiconductor quantum dot and the resulting dephasing of heavy-hole spin states. It has frequently been stated in the literature that heavy holes have a negligible interaction with nuclear spins. We show that this is not the case. In contrast, the interaction can be rather strong and will be the dominant source of decoherence in some cases. We also show that the form of the interaction is Ising-like, resulting in unique and interesting decoherence properties, which might provide a crucial advantage to using dot-confined hole spins for quantum information processing, as compared to electron spins.

We investigate mesoscopic fluctuations in the spin polarization generated by a static electric field and by Rashba spin-orbit interaction in a disordered 2D electron gas. In a diagrammatic approach we find that the out-of-plane polarization -- while being zero for self-averaging systems -- exhibits large sample-to-sample fluctuations which are shown to be well within experimental reach. We evaluate the disorder-averaged variance of the susceptibility and find its dependence on magnetic field, spin-orbit interaction, dephasing, and chemical potential difference.

We study the triangular antiferromagnet Cu$_3$ in external electric fields, using symmetry group arguments and a Hubbard model approach. We identify a spin-electric coupling caused by an interplay between spin exchange, spin-orbit interaction, and the chirality of the underlying spin texture of the molecular magnet. This coupling allows for the electric control of the spin (qubit) states, e.g. by using an STM tip or a microwave cavity. We propose an experimental test for identifying molecular magnets exhibiting spin-electric effects.

We investigate the ac transport of magnetization in non-itinerant quantum systems such as spin chains described by the XXZ Hamiltonian. Using linear response theory, we calculate the ac magnetization current and the power absorption of such magnetic systems. Remarkably, the difference in the exchange interaction of the spin chain itself and the bulk magnets (i.e. the magnetization reservoirs), to which the spin chain is coupled, strongly influences the absorbed power of the system. This feature can be used in future spintronic devices to control power dissipation. Our analysis allows to make quantitative predictions about the power absorption and we show that magnetic systems are superior to their electronic counter parts.

The competition between the Zeeman energy and the Rashba and Dresselhaus spin-orbit couplings is studied for fractional quantum Hall states by including correlation effects. A transition of the direction of the spin-polarization is predicted at specific values of the Zeeman energy. We show that these values can be expressed in terms of the pair-correlation function, which thus provides a way to obtain experimental access to the corresponding ground state. As specific examples, we consider the Laughlin wavefunctions and the 5/2-Pfaffian state and find indications of non-analytic features around the fractional states. We also include effects of the nuclear bath, becoming relevant in the mK-regime.

We show how to map a given n-qubit target Hamiltonian with bounded-strength k-body interactions onto a simulator Hamiltonian with two-body interactions, such that the ground-state energy of the target and the simulator Hamiltonians are the same up to an extensive error O(epsilon n) for arbitrary small epsilon. The strength of interactions in the simulator Hamiltonian depends on epsilon and k but does not depend on n. We accomplish this reduction using a new way of deriving an effective low-energy Hamiltonian which relies on the Schrieffer-Wolff transformation of many-body physics.

We analyze nuclear spin dynamics in quantum dots and defect centers with a bound electron under electron-mediated coupling between nuclear spins due to the hyperfine interaction ("J-coupling" in NMR). Our analysis shows that the Overhauser field generated by the nuclei at the position of the electron has short-time dynamics quadratic in time for an initial nuclear spin state without transverse coherence. The quadratic short-time behavior allows for an extension of the Overhauser field lifetime through a sequence of projective measurements (quantum Zeno effect). We analyze the requirements on the repetition rate of measurements and the measurement accuracy to achieve such an effect. Further, we calculate the long-time behavior of the Overhauser field for effective electron Zeeman splittings larger than the hyperfine coupling strength and find, both in a Dyson series expansion and a generalized master equation approach, that for a nuclear spin system with a sufficiently smooth polarization the electron-mediated interaction alone leads only to a partial decay of the Overhauser field by an amount on the order of the inverse number of nuclear spins interacting with the electron.

We study spin relaxation and decoherence caused by electron-lattice and spin-orbit interaction and predict striking effects induced by magnetic fields B. For particular values of B, destructive interference occurs resulting in ultralong spin relaxation times T1 exceeding tens of seconds. For small phonon frequencies \omega, we find a 1/\sqrt{\omega} spin-phonon noise spectrum --a novel dissipation channel for spins in quantum dots --which can reduce T1 by many orders of magnitude. We show that nanotubes exhibit zero-field level splitting caused by spin-orbit interaction. This enables an all-electrical and phase-coherent control of spin.

We show that the coherence of an electron spin interacting with a bath of nuclear spins can exhibit a well-defined purely exponential decay for special (`narrowed') bath initial conditions in the presence of a strong applied magnetic field. This is in contrast to the typical case, where spin-bath dynamics have been investigated in the non-Markovian limit, giving super-exponential or power-law decay of correlation functions. We calculate the relevant decoherence time T_2 explicitly for free-induction decay and find a simple expression with dependence on bath polarization, magnetic field, the shape of the electron wave function, dimensionality, total nuclear spin I, and isotopic concentration for experimentally relevant heteronuclear spin systems.

We investigate the magnetic behavior of nuclear spins embedded in a 2D interacting electron gas using a Kondo lattice model description. We derive an effective magnetic Hamiltonian for the nuclear spins which is of the RKKY type and where the interactions between the nuclear spins are strongly modified by the electron-electron interactions. We show that the nuclear magnetic ordering at finite temperature relies on the (anomalous) behavior of the 2D static electron spin susceptibility, and thus provides a connection between low-dimensional magnetism and non-analyticities in interacting 2D electron systems. Using various perturbative and non-perturbative approximation schemes in order to establish the general shape of the electron spin susceptibility as function of its wave vector, we show that the nuclear spins locally order ferromagnetically, and that this ordering can become global in certain regimes of interest. We demonstrate that the associated Curie temperature for the nuclear system increases with the electron-electron interactions up to the millikelvin range.

We show that the conductivity tensor of a disordered two-dimensional electron gas becomes anisotropic in the presence of both Rashba and Dresselhaus spin-orbit interactions (SOI). This anisotropy is a mesoscopic effect and vanishes with vanishing charge dephasing time. Using a diagrammatic approach including zero, one, and two-loop diagrams, we show that a consistent calculation needs to go beyond a Boltzmann equation approach. In the absence of charge dephasing and for zero frequency, a finite anisotropy \sigma_xy~ e^2/lhpf arises even for infinitesimal SOI.

We study theoretically electron spins in nanowire quantum dots placed inside a transmission line resonator. Because of the spin-orbit interaction, the spins couple to the electric component of the resonator electromagnetic field and enable coherent manipulation, storage, and read-out of quantum information in an all-electrical fashion. Coupling between distant quantum-dot spins, in one and the same or different nanowires, can be efficiently performed via the resonator mode either in real time or through virtual processes. For the latter case we derive an effective spin-entangling interaction and suggest means to turn it on and off. We consider both transverse and longitudinal types of nanowire quantum-dots and compare their manipulation timescales against the spin relaxation times. For this, we evaluate the rates for spin relaxation induced by the nanowire vibrations (phonons) and show that, as a result of phonon confinement in the nanowire, this rate is a strongly varying function of the spin operation frequency and thus can be drastically reduced compared to lateral quantum dots in GaAs. Our scheme is a step forward to the formation of hybrid structures where qubits of different nature can be integrated in a single device.

We discuss a measurement-based implementation of a Controlled-NOT (CNOT) quantum gate. Such a gate has recently been discussed for free electron qubits. Here we extend this scheme for qubits encoded in product states of two (or more) spins-1/2 or in equivalent systems. The key to such an extension is to find a feasible qubit-parity meter. We present a general scheme for reducing this meter to a local spin-parity measurement performed on two spins, one from each qubit. Two possible realizations of a multi-particle CNOT are further discussed: Electron spins in double quantum dots in the singlet-triplet encoding and nu=5/2 Ising non-Abelian anyons using topological quantum computation braiding operations and nontopological charge measurements.

We describe an algorithm that computes the ground state energy and correlation functions for 2-local Hamiltonians in which interactions between qubits are weak compared to single-qubit terms. The running time of the algorithm is polynomial in the number of qubits and the required precision. Specifically, we consider Hamiltonians of the form $H=H_0+\epsilon V$, where H_0 describes non-interacting qubits, V is a perturbation that involves arbitrary two-qubit interactions on a graph of bounded degree, and $\epsilon$ is a small parameter. The algorithm works if $|\epsilon|$ is below a certain threshold value that depends only upon the spectral gap of H_0, the maximal degree of the graph, and the maximal norm of the two-qubit interactions. The main technical ingredient of the algorithm is a generalized Kirkwood-Thomas ansatz for the ground state. The parameters of the ansatz are computed using perturbative expansions in powers of $\epsilon$. Our algorithm is closely related to the coupled cluster method used in quantum chemistry.

In this article we review our work on the dynamics and decoherence of electron and hole spins in single and double quantum dots. The first part, on electron spins, focuses on decoherence induced via the hyperfine interaction while the second part covers decoherence and relaxation of heavy-hole spins due to spin-orbit interaction as well as the manipulation of heavy-hole spin using electric dipole spin resonance.

We review recent advances on the theory of spin qubits in nanostructures. We focus on four selected topics. First, we show how to form spin qubits in the new and promising material graphene. Afterwards, we discuss spin relaxation and decoherence in quantum dots. In particular, we demonstrate how charge fluctations in the surrounding environment cause spin decay via spin--orbit coupling. We then turn to a brief overview of how one can use electron-dipole spin resonance (EDSR) to perform single spin rotations in quantum dots using an oscillating electric field. The final topic we cover is the spin-spin coupling via spin-orbit interaction which is an alternative to the usual spin-spin coupling via the Heisenberg exchange interaction.

We investigate the creation of highly entangled ground states in a system of three exchange-coupled qubits arranged in a ring geometry. Suitable magnetic field configurations yielding approximate GHZ and exact W ground states are identified. The entanglement in the system is studied at finite temperature in terms of the mixed-state tangle tau. By adapting a steepest-descent optimization algorithm we demonstrate that tau can be evaluated efficiently and with high precision. We identify the parameter regime for which the equilibrium entanglement of the tripartite system reaches its maximum.

Spin qubits offer one of the most promising routes to the implementation of quantum computers. Very recent results in semiconductor quantum dots show that electrically-controlled gating schemes are particularly well-suited for the realization of a universal set of quantum logical gates. Scalability to a larger number of qubits, however, remains an issue for such semiconductor quantum dots. In contrast, a chemical bottom-up approach allows one to produce identical units in which localized spins represent the qubits. Molecular magnetism has produced a wide range of systems with tailored properties, but molecules permitting electrical gating have been lacking. Here we propose to use the polyoxometalate [PMo12O40(VO)2]q-, where two localized spins-1/2 can be coupled through the electrons of the central core. Via electrical manipulation of the molecular redox potential, the charge of the core can be changed. With this setup, two-qubit gates and qubit readout can be implemented.

We report the measurement of extremely slow hole spin relaxation dynamics in self-assembled InGaAs quantum dots. Individual spin orientated holes are optically created in the lowest orbital state of each dot and read out after a defined storage time using spin memory devices. The hole spin relaxation time (T_1h) is measured as a function of the external magnetic field and lattice temperature. As predicted by theory, hole spin relaxation can occur over remarkably long timescales in strongly confined quantum dots (up to T_1h ~270 \mus) comparable to the corresponding time for electrons. Our findings are supported by calculations that reproduce both the observed magnetic field and temperature dependencies. The results show that hole spin relaxation in strongly confined quantum dots is governed by spin-lattice interaction, in marked contrast to higher dimensional nanostructures where it is limited by spin-orbit coupling between valence bands.

Electrons in a two-dimensional semiconducting heterostructure interact with nuclear spins via the hyperfine interaction. Using a a Kondo lattice formulation of the electron-nuclear spin interaction, we show that the nuclear spin system within an interacting two-dimensional electron gas undergoes a ferromagnetic phase transition at finite temperatures. We find that electron-electron interactions and non-Fermi liquid behavior substantially enhance the nuclear spin Curie temperature into the $mK$ range with decreasing electron density.

We study, both theoretically and experimentally, driven Rabi oscillations of a single electron spin coupled to a nuclear spin bath. Due to the long correlation time of the bath, two unusual features are observed in the oscillations. The decay follows a power law, and the oscillations are shifted in phase by a universal value of ~pi/4. These properties are well understood from a theoretical expression that we derive here in the static limit for the nuclear bath. This improved understanding of the coupled electron-nuclear system is important for future experiments using the electron spin as a qubit.

We study spin relaxation in a two-electron quantum dot in the vicinity of the singlet-triplet transition. The spin relaxation occurs due to a combined effect of the spin-orbit, Zeeman, and electron-phonon interactions. The singlet-triplet relaxation rates exhibit strong variations as a function of the singlet-triplet splitting. We show that the Coulomb interaction between the electrons has two competing effects on the singlet-triplet spin relaxation. One effect is to enhance the relative strength of spin-orbit coupling in the quantum dot, resulting in larger spin-orbit splittings and thus in a stronger coupling of spin to charge. The other effect is to make the charge density profiles of the singlet and triplet look similar to each other, thus diminishing the ability of charge environments to discriminate between singlet and triplet states. We thus find essentially different channels of singlet-triplet relaxation for the case of strong and weak Coulomb interaction. Finally, for the linear in momentum Dresselhaus and Rashba spin-orbit interactions, we calculate the singlet-triplet relaxation rates to leading order in the spin-orbit interaction, and find that they are proportional to the second power of the Zeeman energy, in agreement with recent experiments on triplet-to-singlet relaxation in quantum dots.

We consider electrical transport through molecules with Heisenberg-coupled spins arranged in a ring structure in the presence of an easy-axis anisotropy. The molecules are coupled to two metallic leads and a gate. In the charged state of the ring, a Zener double-exchange mechanism links transport properties to the underlying spin structure. This leads to a remarkable contact-site dependence of the current, which for an antiferromagnetic coupling of the spins can lead to a total suppression of the zero-bias conductance when the molecule is contacted at adjacent sites.

We propose how to form spin qubits in graphene. A crucial requirement to achieve this goal is to find quantum dot states where the usual valley degeneracy in bulk graphene is lifted. We show that this problem can be avoided in quantum dots based on ribbons of graphene with semiconducting armchair boundaries. For such a setup, we find the energies and the exact wave functions of bound states, which are required for localized qubits. Additionally, we show that spin qubits in graphene can not only be coupled between nearest neighbor quantum dots via Heisenberg exchange interaction but also over long distances. This remarkable feature is a direct consequence of the quasi-relativistic spectrum of graphene. See also http://www.nature.com/nnano/reshigh/2006/1106/full/nnano.2006.167.html

We show theoretically that arbitrary coherent rotations can be performed quickly (with a gating time ~1 ns) and with high fidelity on the spin of a single electron confined to a quantum dot using exchange. These rotations can be performed using experimentally proven techniques for rapid exchange control, without the need for spin-orbit interaction or ac electromagnetic fields. We expect that implementations of this scheme would achieve gate error rates on the order of $\eta\lesssim 10^-3$, within reach of several known error-correction schemes.

We propose and analyze a new method for manipulation of a heavy hole spin in a quantum dot. Due to spin-orbit coupling between states with different orbital momenta and opposite spin orientations, an applied rf electric field induces transitions between spin-up and spin-down states. This scheme can be used for detection of heavy-hole spin resonance signals, for the control of the spin dynamics in two-dimensional systems, and for determining important parameters of heavy-holes such as the effective $g$-factor, mass, spin-orbit coupling constants, spin relaxation and decoherence times.

We study the spin polarization and its associated spin-Hall current due to EDSR in disordered two-dimensional electron systems. We show that the disorder induced damping of the resonant spin polarization can be strongly reduced by an optimal field configuration that exploits the interference between Rashba and Dresselhaus spin-orbit interaction. This leads to a striking enhancement of the spin susceptibility while the spin-Hall current vanishes at the same time. We give an interpretation of the spin current in geometrical terms which are associated with the trajectories the polarization describes in spin space.

We discuss a few current developments in the use of quantum mechanically coherent systems for information processing. In each of these developments, Rolf Landauer has played a crucial role in nudging us and other workers in the field into asking the right questions, some of which we have been lucky enough to answer. A general overview of the key ideas of quantum error correction is given. We discuss how quantum entanglement is the key to protecting quantum states from decoherence in a manner which, in a theoretical sense, is as effective as the protection of digital data from bit noise. We also discuss five general criteria which must be satisfied to implement a quantum computer in the laboratory, and we illustrate the application of these criteria by discussing our ideas for creating a quantum computer out of the spin states of coupled quantum dots.

We demonstrate control of the electron number down to the last electron in tunable few-electron quantum dots defined in catalytically grown InAs nanowires. Using low temperature transport spectroscopy in the Coulomb blockade regime we propose a simple method to directly determine the magnitude of the spin-orbit interaction in a two-electron artificial atom with strong spin-orbit coupling. Due to a large effective g-factor |g*|=8+/-1 the transition from singlet S to triplet T+ groundstate with increasing magnetic field is dominated by the Zeeman energy rather than by orbital effects. We find that the spin-orbit coupling mixes the T+ and S states and thus induces an avoided crossing with magnitude $\Delta_SO$=0.25+/-0.05 meV. This allows us to calculate the spin-orbit length $\lambda_SO\approx$127 nm in such systems using a simple model.

Recently, we have introduced a novel inter-subband-induced spin-orbit (s-o) coupling (cond-mat/0607218) arising in symmetric wells with at least two subbands. This new s-o coupling gives rise to an usual zitterbewegung -- i.e. the semiconductor analog to the relativistic trembling motion of electrons -- with cycloidal motion without magnetic fields. Here we complement these findings by explicitly deriving expressions for the corresponding zitterbewegung in spin space.

Using canonical transformations we diagonalize approximately the Hamiltonian of a gaussian wire with Rashba spin-orbit interaction. This proceedure allows us to obtain the energy dispersion relations and the wavefunctions with good accuracy, even in systems with relatively strong Rashba coupling. With these eigenstates one can calculate the non-equilibrium spin densities induced by applying bias voltages across the sample. We focus on the $z$-component of the spin density, which is related to the spin Hall effect.

In this article we analyze spin dynamics for electrons confined to semiconductor quantum dots due to the contact hyperfine interaction. We compare mean-field (classical) evolution of an electron spin in the presence of a nuclear field with the exact quantum evolution for the special case of uniform hyperfine coupling constants. We find that (in this special case) the zero-magnetic-field dynamics due to the mean-field approximation and quantum evolution are similar. However, in a finite magnetic field, the quantum and classical solutions agree only up to a certain time scale t<\tau_c, after which they differ markedly.

We investigate a mesoscopic setup composed of a small electron droplet (dot) coupled to a larger quantum dot (grain) also subject to Coulomb blockade as well as two macroscopic leads used as source and drain. An exotic Kondo ground state other than the standard SU(2) Fermi liquid unambiguously emerges: an SU(4) Kondo correlated liquid. The transport properties through the small dot are analyzed for this regime, through boundary conformal field theory, and allow a clear distinction with other regimes such as a two-channel spin state or a two-channel orbital state.

In this review we discuss a recent proposal to perform partial Bell-state (parity) measurements on two-electron spin states for electrons confined to quantum dots. The realization of this proposal would allow for a physical implementation of measurement-based quantum computing. In addition, we consider the primary sources of energy relaxation and decoherence which provide the ultimate limit to all proposals for quantum information processing using electron spins in quantum dots. We give an account of the Hamiltonians used for the most important interactions (spin-orbit and hyperfine) and survey some of the recent work done to understand dynamics, control, and decoherence under the action of these Hamiltonians. We conclude the review with a table of important decay times found in experiment, and relate these time scales to the potential viability of measurement-based quantum computing.

We study the spin-spin coupling between two single-electron quantum dots due to the Coulomb and spin-orbit interactions, in the absence of tunneling between the dots. We find an anisotropic XY spin-spin interaction that is proportional to the Zeeman splitting produced by the external magnetic field. This interaction is studied both in the limit of weak and strong Coulomb repulsion with respect to the level spacing of the dot. The interaction is found to be a non-monotonic function of inter-dot distance $a_0$ and external magnetic field, and, moreover, vanishes for some special values of $a_0$ and/or magnetic field orientation. This mechanism thus provides a new way to generate and tune spin interaction between quantum dots. We propose a scheme to measure this spin-spin interaction based on the spin-relaxation-measurement technique.

We investigate the spin-orbit (s-o) interaction in two-dimensional electron gases (2DEGs) in quantum wells with two subbands. From the $8\times 8$ Kane model, we derive a new inter-subband-induced s-o coupling which resembles the functional form of the Rashba s-o -- but is non-zero even in \emph{symmetric} structures. This follows from the distinct parity of the confined states (even/odd) which obliterates the need for asymmetric potentials. Interestingly, our s-o interaction gives rise to an unusual \emph{zitterbewegung} of spin-polarized electrons with cycloidal trajectories \textit{without} magnetic fields. We also predict a sizable effective-mass renormalization due to the s-o--induced subband warping.

The ability to perform high-precision one- and two-qubit operations is sufficient for universal quantum computation. For the Loss-DiVincenzo proposal to use single electron spins confned to quantum dots as qubits, it is therefore sufficient to analyze only single- and coupled double-dot structures, since the strong Heisenberg exchange coupling between spins in this proposal falls off exponentially with distance and long-ranged dipolar coupling mechanisms can be made significantly weaker. This scalability of the Loss-DiVincenzo design is both a practical necessity for eventual applications of multi-qubit quantum computing and a great conceptual advantage, making analysis of the relevant components relatively transparent and systematic. We review the Loss-DiVincenzo proposal for quantum-dot-confned electron spin qubits, and survey the current state of experiment and theory regarding the relevant single- and double- quantum dots, with a brief look at some related alternative schemes for quantum computing.

We review our investigation of the spin dynamics for two electrons confined to a double quantum dot under the influence of the hyperfine interaction between the electron spins and the surrounding nuclei. Further we propose a scheme to narrow the distribution of difference in polarization between the two dots in order to suppress hyperfine induced decoherence.

We report electrical transport measurements through a semiconducting single-walled carbon nanotube (SWNT) with three additional top-gates. At low temperatures the system acts as a double quantum dot with large inter-dot tunnel coupling allowing for the observation of tunnel-coupled molecular states extending over the whole double-dot system. We precisely extract the tunnel coupling and identify the molecular states by the sequential-tunneling line shape of the resonances in differential conductance.

One of the hallmarks of spintronics is the control of magnetic moments by electric fields enabled by strong spin-orbit interaction (SOI) in semiconductors. A powerful way of manipulating spins in such structures is electric-dipole-induced spin resonance (EDSR), where the radio-frequency fields driving the spins are electric, not magnetic as in standard paramagnetic resonance. Here, we present a theoretical study of EDSR for a two-dimensional electron gas in the presence of disorder, where random impurities not only determine the electric resistance but also the spin dynamics through SOI. Considering a specific geometry with the electric and magnetic fields parallel and in-plane, we show that the magnetization develops an out-of-plane component at resonance that survives the presence of disorder. We also discuss the spin Hall current generated by EDSR. These results are derived in a diagrammatic approach, with the dominant effects coming from the spin vertex correction, and the optimal parameter regime for observation is identified. See also, 'Semiconductor physics: Electric fields drive spins', by Emmanuel I. Rashba, Nature Physics 2, 149-150 (01 Mar 2006) News and Views

An alternating electric field, applied to a ``spin 1/2'' quantum dot, couples to the electron spin via the spin-orbit interaction. We analyze different types of spin-orbit couplings known in the literature and find that an electric dipole spin resonance (EDSR) scheme for spin manipulation can be realized with the up-to-date experimental setups. In particular, for the Rashba and Dresselhaus spin-orbit couplings, a fully transverse effective magnetic field arises in the presence of a Zeeman splitting in the lowest order of spin-orbit interaction. Spin manipulation and measurement of the spin decoherence time $T_2$ are straightforward in lateral GaAs quantum dots through the use of EDSR.

The notion of zitterbewegung is a long-standing prediction of relativistic quantum mechanics. Here we extend earlier theoretical studies on this phenomenon for the case of III-V zinc-blende semiconductors which exhibit particularly strong spin-orbit coupling. This property makes nanostructures made of these materials very favorable systems for possible experimental observations of zitterbewegung. Our investigations include electrons in n-doped quantum wells under the influence of both Rashba and Dresselhaus spin-orbit interaction, and also the two-dimensional hole gas. Moreover, we give a detailed anaysis of electron zitterbewegung in quantum wires which appear to be particularly suited for experimentally observing this effect.

We study a model for a pair of qubits which interact with a single off-resonant cavity mode and, in addition, exhibit a direct inter-qubit coupling. Possible realizations for such a system include coupled superconducting qubits in a line resonator as well as exciton states or electron spin states of quantum dots in a cavity. The emergent dynamical phenomena are strongly dependent on the relative energy scales of the inter-qubit coupling strength, the coupling strength between qubits and cavity mode, and the cavity mode detuning. We show that the cavity mode dispersion enables a measurement of the state of the coupled-qubit system in the perturbative regime. We discuss the effect of the direct inter-qubit interaction on a cavity-mediated two-qubit gate. Further, we show that for asymmetric coupling of the two qubits to the cavity, the direct inter-qubit coupling can be controlled optically via the ac Stark effect.

We theoretically introduce a mesoscopic pendulum from a triple dot. The pendulum is fastened through a singly-occupied dot (spin qubit). Two other strongly capacitively coupled islands form a double-dot charge qubit with one electron in excess oscillating between the two low-energy charge states (1, 0) and (0, 1). The triple dot is placed between two superconducting leads. Under realistic conditions, the main proximity effect stems from the injection of resonating singlet (valence) bonds on the triple dot. This gives rise to a Josephson current that is charge- and spin-dependent and, as a consequence, exhibits a distinct resonance as a function of the superconducting phase difference.

We consider a mechanism of spin decay for an electron spin in a quantum dot due to coupling to a nearby quantum point contact (QPC) with and without an applied bias voltage. The coupling of spin to charge is induced by the spin-orbit interaction in the presence of a magnetic field. We perform a microscopic calculation of the effective Hamiltonian coupling constants to obtain the QPC-induced spin relaxation and decoherence rates in a realistic system. This rate is shown to be proportional to the shot noise of the QPC in the regime of large bias voltage and scales as $a^-6$ where $a$ is the distance between the quantum dot and the QPC. We find that, for some specific orientations of the setup with respect to the crystallographic axes, the QPC-induced spin relaxation and decoherence rates vanish, while the charge sensitivity of the QPC is not changed. This result can be used in experiments to minimize QPC-induced spin decay in read-out schemes.

We study spin dynamics for two electrons confined to a double quantum dot under the influence of an oscillating exchange interaction. This leads to driven Rabi oscillations between the $\ket{\uparrow\downarrow}$--state and the $\ket{\downarrow\uparrow}$--state of the two--electron system. The width of the Rabi resonance is proportional to the amplitude of the oscillating exchange. A measurement of the Rabi resonance allows one to narrow the distribution of nuclear spin states and thereby to prolong the spin decoherence time. Further, we study decoherence of the two-electron states due to the hyperfine interaction and give requirements on the parameters of the system in order to initialize in the $\ket{\uparrow\downarrow}$--state and to perform a $\sqrt{\mathrm{SWAP}}$ operation with unit fidelity.

We consider cotunneling through a quantum dot in the presence of spin-flip processes induced by the coupling to acoustic phonons of the surrounding. An expression for the phonon-assisted cotunneling current is derived by means of a generalized Schrieffer-Wolff transformation. The influence of the spin-phonon coupling on the heating of the dot is considered. The result is evaluated for the case of a parabolic semiconductor quantum dot with Rashba and Dresselhaus spin-orbit coupling and a novel method for the determination of the spin-phonon relaxation rate is proposed.

We extend our previous work on shot noise for entangled and spin polarized electrons in a beam-splitter geometry with spin-orbit (\textit{s-o}) interaction in one of the incoming leads (lead 1). Besides accounting for both the Dresselhaus and the Rashba spin-orbit terms, we present general formulas for the shot noise of singlet and triplets states derived within the scattering approach. We determine the full scattering matrix of the system for the case of leads with \textit{two} orbital channels coupled via weak \textit{s-o} interactions inducing channel anticrossings. We show that this interband coupling coherently transfers electrons between the channels and gives rise to an additional modulation angle -- dependent on both the Rashba and Dresselhaus interaction strengths -- which allows for further independent coherent control of the electrons traversing the incoming leads. We derive explicit shot noise formulas for a variety of correlated pairs (e.g., Bell states) and lead spin polarizations. Interestingly, the singlet and \textit{each} of the triplets defined along the quantization axis perpendicular to lead 1 (with the local \textit{s-o} interaction) and in the plane of the beam splitter display distinctive shot noise for injection energies near the channel anticrossings; hence, one can tell apart all the triplets, in addition to the singlet, through noise measurements. We also find that spin-orbit induced backscattering within lead 1 reduces the visibility of the noise oscillations, due to the additional partition noise in this lead. Finally, we consider injection of two-particle wavepackets into leads with multiple discrete states and find that two-particle entanglement can still be observed via noise bunching and antibunching.

We present an excerpt of the document "Quantum Information Processing and Communication: Strategic report on current status, visions and goals for research in Europe", which has been recently published in electronic form at the website of FET (the Future and Emerging Technologies Unit of the Directorate General Information Society of the European Commission, http://www.cordis.lu/ist/fet/qipc-sr.htm). This document has been elaborated, following a former suggestion by FET, by a committee of QIPC scientists to provide input towards the European Commission for the preparation of the Seventh Framework Program. Besides being a document addressed to policy makers and funding agencies (both at the European and national level), the document contains a detailed scientific assessment of the state-of-the-art, main research goals, challenges, strengths, weaknesses, visions and perspectives of all the most relevant QIPC sub-fields, that we report here.

We propose a protocol and physical implementation for partial Bell-state measurements of Fermionic qubits, allowing for deterministic quantum computing in solid-state systems without the need for two-qubit gates. Our scheme consists of two spin qubits in a double quantum dot where the two dots have different Zeeman splittings and resonant tunneling between the dots is only allowed when the spins are antiparallel. This converts spin parity into charge information by means of a projective measurement and can be implemented with established technologies. This measurement-based qubit scheme greatly simplifies the experimental realization of scalable quantum computers in electronic nanostructures.

Two quantum dots with tunable mutual tunnel coupling have been embedded in a two-terminal Aharonov-Bohm geometry. Aharonov-Bohm oscillations are investigated in the cotunneling regime. Visibilities of more than 0.8 are measured indicating that phase-coherent processes are involved in the elastic and inelastic cotunneling. An oscillation-phase change of pi is detected as a function of bias voltage at the inelastic cotunneling onset.

We have evaluated hyperfine-induced electron spin dynamics for two electrons confined to a double quantum dot. Our quantum solution accounts for decay of a singlet-triplet correlator even in the presence of a fully static nuclear spin system, with no ensemble averaging over initial conditions. In contrast to an earlier semiclassical calculation, which neglects the exchange interaction, we find that the singlet-triplet correlator shows a long-time saturation value that differs from 1/2, even in the presence of a strong magnetic field. Furthermore, we find that the form of the long-time decay undergoes a transition from a rapid Gaussian to a slow power law ($\sim 1/t^3/2$) when the exchange interaction becomes nonzero and the singlet-triplet correlator acquires a phase shift given by a universal (parameter independent) value of $3\pi/4$ at long times. The oscillation frequency and time-dependent phase shift of the singlet-triplet correlator can be used to perform a precision measurement of the exchange interaction and Overhauser field fluctuations in an experimentally accessible system. We also address the effect of orbital dephasing on singlet-triplet decoherence, and find that there is an optimal operating point where orbital dephasing becomes negligible.

We derive analytical expressions for the quasiparticle lifetime \tau, the effective mass m^*, and the Green's function renormalization factor Z for a 2D Fermi liquid with electron-electron interaction in the presence of the Rashba spin-orbit interaction. For the lifetime \tau and the renormalization Z, we find that the modification is independent of the Rashba band index \rho, and occurs in second order of the spin-orbit coupling \alpha . On the contrary, the modification of the effective mass m^* is linear in \alpha and is different for the two Rashba bands, yielding a spin-dependent effective mass. In the derivation of these results, we also discuss the screening of the Coulomb interaction, and the susceptibility.

We study the zitterbewegung of electronic wave packets in III-V zinc-blende semiconductor quantum wells due to spin-orbit coupling. Our results suggest a direct experimental proof of this fundamental effect, confirming a long-standing theoretical prediction. For electron motion in a harmonic quantum wire, we numerically and analytically find a resonance condition maximizing the zitterbewegung. See also, 'Dirac gets the jitters', M. Buchanan, Nature Physics 1, 5 (2005); http://www.nature.com/nphys/journal/v1/n1/full/nphys132.html

We propose a scheme where transport measurements of charge current and its noise can be used to determine the spin Hall conductance in a four-terminal setup. Starting from the scattering formalism we express the spin current and spin Hall conductance in terms of spin-dependent transmission coefficients. These coefficients are then expressed in terms of charge current and noise. We use the scheme to characterize the spin injection efficiency of a ferromagnetic/semiconductor interface.

We investigate heavy-hole spin relaxation and decoherence in quantum dots in perpendicular magnetic fields. We show that at low temperatures the spin decoherence time is two times longer than the spin relaxation time. We find that the spin relaxation time for heavy holes can be comparable to or even longer than that for electrons in strongly two-dimensional quantum dots. We discuss the difference in the magnetic-field dependence of the spin relaxation rate due to Rashba or Dresselhaus spin-orbit coupling for systems with positive (i.e., GaAs quantum dots) or negative (i.e., InAs quantum dots) $g$-factor.

A detailed investigation of the unusual dynamics of the magnetization of (Et4N)3Fe2F9 (Fe2), containing isolated [Fe2F9]3- dimers, is presented and discussed. Fe2 possesses an S=5 ground state with an energy barrier of 2.40 K due to an axial anisotropy. Poor thermal contact between sample and bath leads to a phonon bottleneck situation, giving rise to butterfly-shaped hysteresis loops below 5 K concomitant with slow decay of the magnetization for magnetic fields Hz applied along the Fe--Fe axis. The butterfly curves are reproduced using a microscopic model based on the interaction of the spins with resonant phonons. The phonon bottleneck allows for the observation of resonant quantum tunneling of the magnetization at 1.8 K, far above the blocking temperature for spin-phonon relaxation. The latter relaxation is probed by AC magnetic susceptibility experiments at various temperatures and bias fields. At H=0, no out-of-phase signal is detected, indicating that at T smaller than 1.8 K Fe2 does not behave as a single-molecule magnet. At 1 kG, relaxation is observed, occurring over the barrier of the thermally accessible S=4 first excited state that forms a combined system with the S=5 state.

Technological growth in the electronics industry has historically been measured by the number of transistors that can be crammed onto a single microchip. Unfortunately, all good things must come to an end; spectacular growth in the number of transistors on a chip requires spectacular reduction of the transistor size. For electrons in semiconductors, the laws of quantum mechanics take over at the nanometre scale, and the conventional wisdom for progress (transistor cramming) must be abandoned. This realization has stimulated extensive research on ways to exploit the spin (in addition to the orbital) degree of freedom of the electron, giving birth to the field of spintronics. Perhaps the most ambitious goal of spintronics is to realize complete control over the quantum mechanical nature of the relevant spins. This prospect has motivated a race to design and build a spintronic device capable of complete control over its quantum mechanical state, and ultimately, performing computations: a quantum computer.
In this tutorial we summarize past and very recent developments which point the way to spin-based quantum computing in the solid-state. After introducing a set of basic requirements for any quantum computer proposal, we offer a brief summary of some of the many theoretical proposals for solid-state quantum computers. We then focus on the Loss-DiVincenzo proposal for quantum computing with the spins of electrons confined to quantum dots. There are many obstacles to building such a quantum device. We address these, and survey recent theoretical, and then experimental progress in the field. To conclude the tutorial, we list some as-yet unrealized experiments, which would be crucial for the development of a quantum-dot quantum computer.

We consider the spin-Hall current in a disordered two-dimensional electron gas in the presence of Rashba spin-orbit interaction. We derive a generalized Kubo-Greenwood formula for the spin-Hall conductivity $\sigma$ and evaluate it in an systematic way using standard diagrammatic techniques for disordered systems. We find that in the diffusive regime both Boltzmann and the weak localization contributions to the $\sigma$ vanish in the zero frequency limit. We show that the uniform spin current is given by the total time derivative of the magnetization from which we can conclude that the spin current vanishes exactly in the stationary limit. This conclusion is valid for arbitrary spin-independent disorder, external electric field strength, and also for interacting electrons.

We show that a special type of entangled states, cluster states, can be created with Heisenberg interactions and local rotations in 2d steps where d is the dimension of the lattice. We find that, by tuning the coupling strengths, anisotropic exchange interactions can also be employed to create cluster states. Finally, we propose electron spins in quantum dots as a possible realization of a one-way quantum computer based on cluster states.

We show that electron recombination in spin light-emitting diodes provides an efficient method to transfer entanglement from electron spins onto pairs of polarization-entangled photons. Because of the interplay of quantum mechanical selection rules and interference, maximally entangled electron pairs are converted into maximally entangled photon pairs with unity fidelity for a continuous set of observation directions. We describe the dynamics of the conversion process using a master-equation approach and show that the implementation of our scheme is feasible with current experimental techniques.

We study the corrections to adiabatic dynamics of two coupled quantum dot spin-qubits, each dot singly occupied with an electron, in the context of a quantum computing operation. Tunneling can lead to a double occupancy at the conclusion of an operation and constitutes a processing error. Our model for the dynamics of an effective two-level system is integrable and possesses three independent parameters. We confirm the accuracy of Dykhne's formula, a nonperturbative estimate of transitions, and discuss physically intuitive conditions for its validity. Our semiclassical results are in excellent agreement with numerical simulations of the exact time evolution. A similar approach applies to two-level systems in different contexts.

The spin-orbit splitting of the electron levels in a two-dimensional quantum dot in a perpendicular magnetic field is studied. It is shown that at the point of an accidental degeneracy of the two lowest levels above the ground state the Rashba spin-orbit coupling leads to a level anticrossing and to mixing of spin-up and spin-down states, whereas there is no mixing of these levels due to the Dresselhaus term. We calculate the relaxation and decoherence times of the three lowest levels due to phonons. We find that the spin relaxation rate as a function of a magnetic field exhibits a cusp-like structure for Rashba but not for Dresselhaus spin-orbit interaction.

We review progress on the spintronics proposal for quantum computing where the quantum bits (qubits) are implemented with electron spins. We calculate the exchange interaction of coupled quantum dots and present experiments, where the exchange coupling is measured via transport. Then, experiments on single spins on dots are described, where long spin relaxation times, on the order of a millisecond, are observed. We consider spin-orbit interaction as sources of spin decoherence and find theoretically that also long decoherence times are expected. Further, we describe the concept of spin filtering using quantum dots and show data of successful experiments. We also show an implementation of a read out scheme for spin qubits and define how qubits can be measured with high precision. Then, we propose new experiments, where the spin decoherence time and the Rabi oscillations of single electrons can be measured via charge transport through quantum dots. Finally, all these achievements have promising applications both in conventional and quantum information processing.

Coherent Rabi oscillations between quantum states of superconducting micro-circuits have been observed in a number of experiments, albeit with a visibility which is typically much smaller than unity. Here, we show that the coherent coupling to background charge fluctuators [R.W. Simmonds et al., Phys. Rev. Lett. 93, 077003 (2004)] leads to a significantly reduced visibility if the Rabi frequency is comparable to the coupling energy of micro-circuit and fluctuator. For larger Rabi frequencies, transitions to the second excited state of the superconducting micro-circuit become dominant in suppressing the Rabi oscillation visibility. We also calculate the probability for Bogoliubov quasi-particle excitations in typical Rabi oscillation experiments.

We present electron spin entanglers--devices creating mobile spin-entangled electrons that are spatially separated--where the spin-entanglement in a superconductor present in form of Cooper pairs and in a single quantum dot with a spin singlet groundstate is transported to two spatially separated leads by means of a correlated two-particle tunneling event. The unwanted process of both electrons tunneling into the same lead is suppressed by strong Coulomb blockade effects caused by quantum dots, Luttinger liquid effects or by resistive outgoing leads. In this review we give a transparent description of the different setups, including discussions of the feasibility of the subsequent detection of spin-entanglement via charge noise measurements. Finally, we show that quantum dots in the spin filter regime can be used to perform Bell-type measurements that only require the measurement of zero frequency charge noise correlators.

We propose to use optical detection of magnetic resonance (ODMR) to measure the decoherence time T₂ of a single electron spin in a semiconductor quantum dot. The electron is in one of the spin 1/2 states and a circularly polarized laser can only create an optical excitation for one of the electron spin states due to Pauli blocking. An applied electron spin resonance (ESR) field leads to Rabi spin flips and thus to a modulation of the photoluminescence or, alternatively, of the photocurrent. This allows one to measure the ESR linewidth and the coherent Rabi oscillations, from which the electron spin decoherence can be determined. We study different possible schemes for such an ODMR setup, including cw or pulsed laser excitation.

We calculate the Coulomb scattering amplitude for two electrons injected with opposite momenta in an interacting 2DEG. We include the effect of the Fermi liquid background by solving the 2D Bethe-Salpeter equation for the two-particle Green function vertex, in the ladder and random phase approximations. This result is used to discuss the feasibility of producing spin EPR pairs in a 2DEG by collecting electrons emerging from collisions at a pi/2 scattering angle, where only the entangled spin-singlets avoid the destructive interference resulting from quantum indistinguishability. Furthermore, we study the effective 2D electron-electron interaction due to the exchange of virtual acoustic and optical phonons, and compare it to the Coulomb interaction. Finally, we show that the 2D Kohn-Luttinger pairing instability for the scattering electrons is negligible in a GaAs 2DEG.

We calculate the frequency dependent spin susceptibilities for a two-dimensional electron gas with both Rashba and Dresselhaus spin-orbit interaction. The resonances of the susceptibilities depends on the relative values of the Rashba and Dresselhaus spin-orbit constants, which could be manipulated by gate voltages. We derive exact continuity equations, with source terms, for the spin density and use those to connect the spin current to the spin density. In the free electron model the susceptibilities play a central role in the spin dynamics since both the spin density and the spin current are proportional to them.

We have performed a systematic calculation for the non-Markovian dynamics of a localized electron spin interacting with an environment of nuclear spins via the Fermi contact hyperfine interaction. This work applies to an electron in the s -type orbital ground state of a quantum dot or bound to a donor impurity, and is valid for arbitrary polarization p of the nuclear spin system, and arbitrary nuclear spin I in high magnetic fields. In the limit of p=1 and I=1/2, the Born approximation of our perturbative theory recovers the exact electron spin dynamics. We have found the form of the generalized master equation (GME) for the longitudinal and transverse components of the electron spin to all orders in the electron spin--nuclear spin flip-flop terms. Our perturbative expansion is regular, unlike standard time-dependent perturbation theory, and can be carried-out to higher orders. We show this explicitly with a fourth-order calculation of the longitudinal spin dynamics. In zero magnetic field, the fraction of the electron spin that decays is bounded by the smallness parameter \delta=1/p²N, where N is the number of nuclear spins within the extent of the electron wave function. However, the form of the decay can only be determined in a high magnetic field, much larger than the maximum Overhauser field. In general the electron spin shows rich dynamics, described by a sum of contributions with non-exponential decay, exponential decay, and undamped oscillations. There is an abrupt crossover in the electron spin asymptotics at a critical dimensionality and shape of the electron envelope wave function. We propose a scheme that could be used to measure the non-Markovian dynamics using a standard spin-echo technique, even when the fraction that undergoes non-Markovian dynamics is small.

Within the lowest-order Born approximation, we present an exact calculation of the time dynamics of the spin-boson model in the ohmic regime. We observe non-Markovian effects at zero temperature that scale with the system-bath coupling strength and cause qualitative changes in the evolution of coherence at intermediate times of order of the oscillation period. These changes could significantly affect the performance of these systems as qubits. In the biased case, we find a prompt loss of coherence at these intermediate times, whose decay rate is set by $\sqrt{\alpha}$, where $\alpha$ is the coupling strength to the environment. We also explore the calculation of the next order Born approximation: we show that, at the expense of very large computational complexity, interesting physical quantities can be rigorously computed at fourth order using computer algebra, presented completely in an accompanying Mathematica file. We compute the $O(\alpha)$ corrections to the long time behavior of the system density matrix; the result is identical to the reduced density matrix of the equilibrium state to the same order in $\alpha$. All these calculations indicate precision experimental tests that could confirm or refute the validity of the spin-boson model in a variety of systems.

We investigate spin transport of heavy holes in III-V semiconductor quantum wells in the presence of spin-orbit coupling of the Rashba type due to structure-inversion asymmetry. Similarly to the case of electrons, the longitudinal spin conductivity vanishes, whereas the off-diagonal elements of the spin-conductivity tensor are finite giving rise to an intrinsic spin-Hall effect. For a clean system we find a closed expression for the spin-Hall conductivity depending on the length scale of the Rashba coupling and the hole density. In this limit the spin-Hall conductivity is enhanced compared to its value for electron systems, and it vanishes with increasing strength of the impurity scattering. As an aside, we also derive explicit expressions for the Fermi momenta and the densities of holes in the different dispersion branches as a function of the spin-orbit coupling parameter and the total hole density. These results are of relevance for the interpretation of possible Shubnikov-de Haas measurements detecting the Rashba spin splitting.

We propose a setup to generate non-local spin-EPR pairs via pair collisions in a 2D interacting electron gas, based on constructive two-particle interference in the spin singlet channel at the pi/2 scattering angle. We calculate the scattering amplitude via the Bethe-Salpeter equation in the ladder approximation and small r_s limit, and find that the Fermi sea leads to a substantial renormalization of the bare scattering process. From the scattering length we estimate the current of spin-entangled electrons and show that it is within experimental reach.

Time-resolved Faraday rotation has recently demonstrated coherent transfer of electron spin between quantum dots coupled by conjugated molecules. Using a transfer Hamiltonian ansatz for the coupled quantum dots, we calculate the Faraday rotation signal as a function of the probe frequency in a pump-probe setup using neutral quantum dots. Additionally, we study the signal of one spin-polarized excess electron in the coupled dots. We show that, in both cases, the Faraday rotation angle is determined by the spin transfer probabilities and the Heisenberg spin exchange energy. By comparison of our results with experimental data, we find that the transfer matrix element for electrons in the conduction band is of order 0.08 eV and the spin transfer probabilities are of order 10%.

We study spin relaxation and decoherence in a
GaAs quantum dot due to spin-orbit interaction. We derive an effective Hamiltonian which couples the electron spin to phonons or any other fluctuation of the dot potential. We show that the spin decoherence time $T_2$ is as large as the spin relaxation time $T_1$, under realistic conditions. For the Dresselhaus and Rashba spin-orbit couplings, we find that, in leading order, the effective magnetic field can have only fluctuations transverse to the applied magnetic field. As a result, $T_2=2T_1$ for arbitrarily large Zeeman splittings, in contrast to the naively expected case
$T_2\ll T_1$. We show that the spin decay is drastically suppressed for certain magnetic field directions and values of the
Rashba coupling constant. Finally, for the spin coupling to acoustic phonons, we show that
$T_2=2T_1$ for all spin-orbit mechanisms in leading order in the electron-phonon interaction.

We analyze the frequency-dependent noise of a current through a quantum dot which is coupled to Fermi leads and which is in the Coulomb blockade regime. We show that the asymmetric shot noise as function of frequency shows steps and becomes super-Poissonian. This provides experimental access to the quantum fluctuations of the current. We present an exact calculation for a single dot level and a perturbative evaluation of the noise in Born approximation (sequential tunneling regime but without Markov approximation) for the general case of many levels with charging interaction.

We have reconsidered the relevant problem of spin injection across ferromagnet/non-magnetic-semiconductor (FM/NMS) and dilute-magnetic-semiconductor/non-magnetic-semiconductor interfaces, for structures with \textit{finite} magnetic layers (FM or DMS). By using appropriate physical boundary conditions, we find new expressions for the resistances of these structures which are in general different from previous results in the literature. The results obtained can be important for the interpretation of the experimental data in the case of DMS/NMS structures.

We review our recent work towards quantum communication in a solid-state environment with qubits carried by electron spins. We propose three schemes to produce spin-entangled electrons, where the required separation of the partner electrons is achieved via Coulomb interaction. The non-product spin-states originate either from the Cooper pairs found in a superconductor, or in the ground state of a quantum dot with an even number of electrons. In a second stage, we show how spin-entanglement carried by a singlet can be detected in a beam-splitter geometry by an increased (bunching) or decreased (antibunching) noise signal. We also discuss how a local spin-orbit interaction can be used to provide a continuous modulation of the noise as a signature of entanglement. Finally, we review how one can use a quantum dot as a spin- lter, a spin-memory read-out, a probe for single-spin decoherence and ultimately, a single-spin measurement apparatus.

We review and summarize recent theoretical and experimental work on electron spin dynamics in quantum dots and related nanostructures due to hyperfine interaction with surrounding nuclear spins. This topic is of particular interest with respect to several proposals for quantum information processing in solid state systems. Specifically, we investigate the hyperfine interaction of an electron spin confined in a quantum dot in an s-type conduction band with the nuclear spins in the dot. This interaction is proportional to the square modulus of the electron wave function at the location of each nucleus leading to an inhomogeneous coupling, i.e. nuclei in different locations are coupled with different strength. In the case of an initially fully polarized nuclear spin system an exact analytical solution for the spin dynamics can be found. For not completely polarized nuclei, approximation-free results can only be obtained numerically in sufficiently small systems. We compare these exact results with findings from several approximation strategies.

We study transport through a double quantum dot, both in the sequential tunneling and cotunneling regimes. Using a master equation approach, we find that, in the sequential tunneling regime, the differential conductance
$G$ as a function of the bias voltage $\Delta\mu$ has a number of satellite peaks with respect to the main peak of the Coulomb blockade diamond. The position of these peaks is related to the interdot tunnel splitting and the singlet-triplet splitting. We find satellite peaks with both {\em positive} and {\em negative} values of differential conductance for realistic parameter regimes. Relating our theory to a microscopic (Hund-Mulliken) model for the double dot, we find a temperature regime for which the Hubbard ratio (=tunnel coupling over on-site Coulomb repulsion) can be extracted from $G(\Delta\mu)$ in the cotunneling regime. In addition, we consider a combined effect of cotunneling and sequential tunneling, which leads to new peaks (dips) in $G(\Delta\mu)$ inside the Coulomb blockade diamond below some temperature scales, which we specify.

We have recently calculated shot noise for entangled and spin-polarized electrons in novel beam-splitter geometries with a local Rashba s-o interaction in the incoming leads. This interaction allows for a gate-controlled rotation of the incoming electron spins. Here we present an alternate simpler route to the shot noise calculation in the above work and focus on only electron pairs. Shot noise for these shows continuous bunching and antibunching behaviors. In addition, entangled and unentangled triplets yield distinctive shot noise oscillations. Besides allowing for a direct way to identify triplet and singlet states, these oscillations can be used to extract s-o coupling constants through noise measurements. Incoming leads with spin-orbit interband mixing give rise an additional modulation of the current noise. This extra rotation allows the design of a spin transistor with enhanced spin control.

We show a possible way to implement the Grover algorithm in large nuclear spins 1/2<I<9/2 in semiconductors. The Grover sequence is performed by means of multiphoton transitions that distribute the spin amplitude between the nuclear spin states. They are distinguishable due to the quadrupolar splitting, which makes the nuclear spin levels non-equidistant. We introduce a generalized rotating frame for an effective Hamiltonian that governs the non-perturbative time evolution of the nuclear spin states for arbitrary spin lengths I. The larger the quadrupolar splitting, the better the agreement between our approximative method using the generalized rotating frame and exact numerical calculations.

We investigate the spin-Hall effect of both electrons and holes in semiconductors using the Kubo formula in the correct zero-frequency limit taking into account the finite momentum relaxation time of carriers in real semiconductors. This approach allows to analyze the range of validity of recent theoretical findings. In particular, the spin-Hall conductivity vanishes for vanishing spin-orbit coupling if the correct zero-frequency limit is performed.

We consider electron spin qubits in quantum dots and define a measurement efficiency e to characterize reliable measurements via n-shot read outs. We propose various implementations based on a double dot and quantum point contact (QPC) and show that the associated efficiencies e vary between 50% and 100%, allowing single-shot read out in the latter case. We model the read out microscopically and derive its time dynamics in terms of a generalized master equation, calculate the QPC current and show that it allows spin read out under realistic conditions.

We consider the production of mobile and nonlocal pairwise spin-entangled electrons from tunneling of a BCS-superconductor (SC) to two normal Fermi liquid leads. The necessary mechanism to separate the two electrons coming from the same Cooper pair (spin-singlet) is achieved by coupling the SC to leads with a finite resistance. The resulting dynamical Coulomb blockade effect, which we describe phenomenologically in terms of an electromagnetic environment, is shown to be enhanced for tunneling of two spin-entangled electrons into the same lead compared to the process where the pair splits and each electron tunnels into a different lead. On the other hand in the pair-split process, the spatial correlation of a Cooper pair leads to a current suppression as a function of distance between the two tunnel junctions which is weaker for effectively lower dimensional SCs.

We propose a method based on optically detected magnetic resonance (ODMR) to measure the decoherence time $T₂$ of a single electron spin in a semiconductor quantum dot. The electron spin resonance (ESR) of a single excess electron on a quantum dot is probed by circularly polarized laser excitation. The photoluminescence is modulated due to the ESR which enables the measurement of electron spin decoherence. We study different possible schemes for such an ODMR setup.

In a two-dimensional electron gas as realized by a semiconductor quantum well, the presence of spin-orbit coupling of both the Rashba and Dresselhaus type leads to anisotropic dispersion relations and Fermi contours. We study the effect of this anisotropy on the electrical conductivity in the presence of fixed impurity scatterers. The conductivity also shows in general an anisotropy which can be tuned by varying the Rashba coefficient. This effect provides a method of detecting and investigating spin-orbit coupling by measuring spin-unpolarized electrical currents in the diffusive regime. Our approach is based on an exact solution of the two-dimensional Boltzmann equation and provides also a natural framework for investigating other transport effects including the anomalous Hall effect.

We show that a wide range of spin clusters with antiferromagnetic intracluster exchange interaction allows one to define a qubit. For these spin cluster qubits, initialization, quantum gate operation, and readout are possible using the same techniques as for single spins. Quantum gate operation for the spin cluster qubit does not require control over the intracluster exchange interaction. Electric and magnetic fields necessary to effect quantum gates need only be controlled on the length scale of the spin cluster rather than the scale for a single spin. Here, we calculate the energy gap separating the logical qubit states from the next excited state and the matrix elements which determine quantum gate operation times. We discuss spin cluster qubits formed by one- and two-dimensional arrays of s=1/2 spins as well as clusters formed by spins s>1/2. We illustrate the advantages of spin cluster qubits for various suggested implementations of spin qubits and analyze the scaling of decoherence time with spin cluster size.

We show that a wide range of spin clusters with antiferromagnetic intracluster exchange interaction allows one to define a qubit. For these spin cluster qubits, initialization, quantum gate operation, and readout are possible using the same techniques as for single spins. Quantum gate operation for the spin cluster qubit does not require control over the intracluster exchange interaction. Electric and magnetic fields necessary to effect quantum gates need only be controlled on the length scale of the spin cluster rather than the scale for a single spin. Here, we calculate the energy gap separating the logical qubit states from the next excited state and the matrix elements which determine quantum gate operation times. We discuss spin cluster qubits formed by one- and two-dimensional arrays of s = 1/2 spins as well as clusters formed by spins s > 1/2. We illustrate the advantages of spin cluster qubits for various suggested implementations of spin qubits and analyze the scaling of decoherence time with spin cluster size.

Within the lowest-order Born approximation, we present an exact calculation of the time dynamics of the spin-boson model in the Ohmic regime. We observe non-Markovian effects at zero temperature that scale with the system-bath coupling strength and cause qualitative changes in the evolution of coherence at intermediate times of order of the oscillation period. These changes could significantly affect the performance of these systems as qubits. In the biased case, we find a prompt loss of coherence at these intermediate times, whose decay rate is set by $\sqrt{\alpha}$, where $\alpha$ is the coupling strength to the environment. These calculations indicate precision experimental tests that could confirm or refute the validity of the spin-boson model in a variety of systems.

We review our recent contributions on shot noise for entangled electrons and spin-polarized currents in novel mesoscopic geometries. We first discuss some of our recent proposals for electron entanglers involving a superconductor coupled to a double dot in the Coulomb blockade regime, a superconductor tunnel-coupled to Luttinger-liquid leads, and a triple-dot setup coupled to Fermi leads. We calculate current and shot noise for spin-polarized currents and entangled/unentangled electron pairs in a beam-splitter geometry with a \textit{local} Rashba spin-orbit (s-o) interaction in the incoming leads. We find \textit{continuous} bunching and antibunching behaviors for the \textit{entangled} pairs -- triplet and singlet -- as a function of the Rashba rotation angle. In addition, we find that unentangled triplets and the entangled one exhibit distinct shot noise. Shot noise for spin-polarized currents shows sizable oscillations as a function of the Rashba phase. This happens only for electrons injected perpendicular to the Rashba rotation axis; spin-polarized carriers along the Rashba axis are noiseless. We find an additional spin rotation for electrons with energies near the crossing of the bands where s-o induced interband coupling is relevant. This gives rise to an additional modulation of the noise for both electron pairs and spin-polarized currents. Finally, we briefly discuss shot noise for a double dot near the Kondo regime.

We study the effect of spin-orbit coupling on quantum gates produced by pulsing the exchange interaction between two single electron quantum dots. Spin-orbit coupling enters as a small spin precession when electrons tunnel between dots. For adiabatic pulses the resulting gate is described by a unitary operator acting on the four-dimensional Hilbert space of two qubits. If the precession axis is fixed, time-symmetric pulsing constrains the set of possible gates to those which, when combined with single qubit rotations, can be used in a simple CNOT construction. Deviations from time-symmetric pulsing spoil this construction. The effect of time asymmetry is studied by numerically integrating the Schr\"odinger equation using parameters appropriate for GaAs quantum dots. Deviations of the implemented gate from the desired form are shown to be proportional to dimensionless measures of both spin-orbit coupling and time asymmetry of the pulse.

The manipulation of electric charge in bulk semiconductors and their heterostructures forms the basis of virtually all contemporary electronic and optoelectronic devices. Recent studies of spin-dependent phenomena in semiconductors have now opened the door to technological possibilities that harness the spin of the electron in semiconductor devices. In addition to providing spin-dependent analogies that extend existing electronic devices into the realm of semiconductor "spintronics" the spin degree of freedom also offers prospects for fundamentally new functionality within the quantum domain, ranging from storage to computation. It is anticipated that the spin degree of freedom in semiconductors will play a crucial role in the development of information technologies in the 21st century. This book brings together a team of experts to provide an overview of emerging concepts in this rapidly developing field. The topics range from spin transport and injection in semiconductors and their heterostructures to coherent processes and quantum computation in semiconductor quantum structures and microcavities.

An electronic beam splitter with a local Rashba spin-orbit coupling can serve as a detector for spin-polarized currents. The spin-orbit coupling plays the role of a tunable spin rotator and can be controlled via a gate electrode on top of the conductor. We use spin-resolved scattering theory to calculate the zero-temperature current fluctuations (shot noise) for such a four-terminal device and show that the shot noise is proportional to the spin polarization of the source. Moreover, we analyze the effect of spin-orbit-induced intersubband coupling, leading to an additional spin rotation.

We determine a lower bound for the entanglement of pairs of electron spins injected into a mesoscopic conductor. The bound can be expressed in terms of experimentally accessible quantities, the zero-frequency current correlators (shot noise power or cross-correlators) after transmission through an electronic beam splitter. The effect of spin relaxation (T_1 processes) and decoherence (T_2 processes) during the ballistic coherent transmission of the carriers in the wires is taken into account within Bloch theory. The presence of a variable inhomogeneous magnetic field allows the determination of a useful lower bound for the entanglement of arbitrary entangled states. The decrease in entanglement due to thermally mixed states is studied. Both the entanglement of the output of a source (entangler) and the relaxation (T_1) and decoherence (T_2) times can be determined.

We study the noise of the cotunneling current through one or several tunnel-coupled quantum dots in the Coulomb blockade regime. The various regimes of weak and strong, elastic and inelastic cotunneling are analyzed for quantum-dot systems (QDS) with few-level, nearly-degenerate, and continuous electronic spectra. In the case of weak cotunneling we prove a non-equilibrium fluctuation-dissipation theorem, which leads to a universal expression for the noise-to-current ratio (Fano factor). The noise of strong inelastic cotunneling can be super-Poissonian due to switching between QDS states carrying currents of different strengths. The transport through a double-dot (DD) system shows an Aharonov-Bohm effect both in noise and current. In the case of cotunneling through a QDS with a continuous energy spectrum the Fano factor is very close to one.

We briefly review the physics of gate operations between quantum dot spin-qubits and analyze the dynamics of quantum entanglement in such processes. The indistinguishable character of the electrons whose spins realize the qubits gives rise to further entanglement-like quantum correlations that go beyond simple antisymmetrization effects. We also summarize further recent results concerning this type of quantum correlations of indistinguishable particles. Finally we discuss decoherence properties of spin-qubits when coupled to surrounding nuclear spins in a semiconductor nanostructure

In this paper we show that the discrete Fourier transform can be performed by scattering a coherent particle or laser beam off a two-dimensional potential that has the shape of rings or peaks. After encoding the initial vector into the two-dimensional potential, the Fourier-transformed vector can be read out by detectors surrounding the potential. The wavelength of the laser beam determines the necessary accuracy of the 2D potential, which makes our method very fault-tolerant.

We study the decoherence of a single electron spin in an isolated quantum dot induced by hyperfine interaction with nuclei for times smaller than the nuclear spin relaxation time. The decay is caused by the spatial variation of the electron envelope wave function within the dot, leading to a non-uniform hyperfine coupling $A$. We show that the usual treatment of the problem based on the Markovian approximation is impossible because the correlation time for the nuclear magnetic field seen by the electron spin is itself determined by the flip-flop processes.
The decay of the electron spin correlation function is not exponential but rather power (inverse logarithm) law-like. For polarized nuclei we find an exact solution and show that the precession amplitude and the decay behavior can be tuned by the magnetic field. The decay time is given by $\hbar N/A$, where $N$ is the number of nuclei inside the dot. The amplitude of precession, reached as a result of the decay, is finite. We show that there is a striking difference between the decoherence time for a single dot and the dephasing time for an ensemble of dots.

Molecular magnetic clusters with antiferromagnetic exchange interaction and easy axis anisotropy belong to the most promising candidate systems for the observation of coherent spin quantum tunneling on the mesoscopic scale. We point out that both nuclear magnetic resonance and electron spin resonance on doped rings are adequate experimental techniques for the detection of coherent spin quantum tunneling in antiferromagnetic molecular rings. Although challenging, the experiments are feasible with present day techniques.

We propose a spin field-effect transistor based on spin-orbit (s-o) coupling of both the Rashba and the Dresselhaus types. Differently from earlier proposals, spin transport through our device is tolerant against spin-independent scattering processes. Hence the requirement of strictly ballistic transport can be relaxed. This follows from a unique interplay between the Dresselhaus and the (gate-controlled) Rashba interactions; these can be tuned to have equal strengths thus yielding k-independent eigenspinors even in two dimensions. We discuss implementations with two-dimensional devices and quantum wires. In the latter, our setup presents strictly parabolic dispersions which avoids complications arising from anticrossings of different bands.

It is remarkable that today's computers, after the tremendous development during the last 50 years, are still essentially described by the mathematical model formulated by Alan Turing in the 1930's. Turing's model describes computers which operate according to the laws of classical physics. What would happen if a computer was operating according to the quantum laws? Physicists and computer scientists have been interested in this question since the early 1980's, but research in quantum computation really started to flourish after 1994 when Peter Shor discovered a quantum algorithm to find prime factors of large integers efficiently, a problem which is intrinsically hard for any classical computer (see [1] for an introduction into quantum computation). The lack of an algorithm for efficient factoring on a classical machine is actually the basis of the widely used RSA encryption scheme. Phase coherence needs to be maintained for a sufficiently long time in the memory of a quantum computer. This may sound like a harmless requirement, but in fact it is the main reason why the physical implementation of quantum computation is so difficult. Usually, a quantum memory is thought of as a set of two-level systems, named quantum bits, or qubits for short. In analogy to the classical bit, two orthogonal computational basis states |0> and |1> are defined. The textbook example of a quantum two-level system is the spin 1/2 of, say, an electron, where one can identify the "spin up" state with |0> and the "spin down" state with |1>. While several other two-level systems have been proposed for quantum computing, we will devote the majority of our discussion to the potential use of electron spins in nanostructures (such as quantum dots) as qubits.

We analyze transport of magnetization in insulating systems described by a spin Hamiltonian. The magnetization current through a quasi one-dimensional magnetic wire of finite length suspended between two bulk magnets is determined by the spin conductance which remains finite in the ballistic limit due to contact resistance. For ferromagnetic systems, magnetization transport can be viewed as transmission of magnons and the spin conductance depends on the temperature T. For antiferromagnetic isotropic spin-1/2 chains, the spin conductance is quantized in units of order $(g \mu_B)^2/h$ at T=0. Magnetization currents produce an electric field and hence can be measured directly. For magnetization transport in electric fields phenomena analogous to the Hall effect emerge.

We consider a two-channel spin transistor with weak spin-orbit induced interband coupling. We show that the coherent transfer of carriers between the coupled channels gives rise to an \textit{additional} spin rotation. We calculate the corresponding spin-resolved current in a Datta-Das geometry and show that a weak interband mixing leads to enhanced spin control.

We investigate the nu=1 quantum Hall ferromagnet in the presence of spin-orbit coupling of the Rashba or Dresselhaus type by means of Hartree-Fock-typed variational states. In the presence of Rashba (Dresselhaus) spin-orbit coupling the fully spin-polarized quantum Hall state is always unstable resulting in a reduction of the spin polarization if the product of the particle charge $q$ and the effective $g$-factor is positive (negative). In all other cases an alternative variational state with O(2) symmetry and finite in-plane spin components is lower in energy than the fully spin-polarized state for large enough spin-orbit interaction. The phase diagram resulting from these considerations differs qualitatively from earlier studies.

We study the time evolution of a single spin coupled inhomogeneously to a spin environment. Such a system is realized by a single electron spin bound in a semiconductor nanostructure and interacting with surrounding nuclear spins. We find striking dependencies on the type of the initial state of the nuclear spin system. Simple product states show a profoundly different behavior than randomly correlated states whose time evolution provides an illustrative example of quantum parallelism and entanglement in a decoherence phenomenon.

We study the low energy states of finite spin chains with isotropic (Heisenberg) and anisotropic (XY and Ising-like) exchange interaction with uniform and non-uniform coupling constants. We show that for an odd number of sites a spin cluster qubit can be defined in terms of the ground state doublet. This qubit is remarkably insensitive to the placement and coupling anisotropy of spins within the cluster. One- and two-qubit quantum gates can be generated by magnetic fields and inter-cluster exchange, and leakage during quantum gate operation is small. Spin cluster qubits inherit the long decoherence times and short gate operation times of single spins. Control of single spins is hence not necessary for the realization of universal quantum gates.

The detailed theoretical understanding of quantum spin dynamics in various molecular magnets is an important step on the roadway to technological applications of these systems. Quantum effects in both ferromagnetic and antiferromagnetic molecular clusters are, by now, theoretically well understood. Ferromagnetic molecular clusters allow one to study the interplay of incoherent quantum tunneling and thermally activated transitions between states with different spin orientation. The Berry phase oscillations found in Fe_8 are signatures of the quantum mechanical interference of different tunneling paths. Antiferromagnetic molecular clusters are promising candidates for the observation of coherent quantum tunneling on the mesoscopic scale. Although challenging, applications of molecular magnetic clusters for data storage and quantum data processing are within experimental reach already with present day technology.

We propose a simple setup of three coupled quantum dots in the Coulomb blockade regime as a source for spatially separated currents of spin-entangled electrons. The entanglement originates from the singlet ground state of a quantum dot with an even number of electrons. To preserve the entanglement of the electron pair during its extraction to the drain leads, the electrons are transported through secondary dots. This prevents one-electron transport by energy mismatch, while joint transport is resonantly enhanced by conservation of the total two-electron energy.

We study shot noise for spin-polarized currents and entangled electron pairs in a four-probe (beam splitter) geometry with a local Rashba spin-orbit (s-o) interaction in the incoming leads. Within the scattering formalism we find that shot noise exhibits Rashba-induced oscillations with continuous bunching and antibunching. We show that entangled states as well as triplet states can be identified via their Rashba phase in noise measurements. For two-channel leads we find an additional spin rotation due to s-o induced interband coupling which provides additional spin control. We show that the s-o interaction determines the Fano factor which provides a direct way to measure the Rashba coupling constant via noise.

We propose an implementation for quantum information processing based on coherent manipulations of nuclear spins I=3/2 in GaAs semiconductors. We describe theoretically an NMR method which involves multiphoton transitions and which exploits the non-equidistance of nuclear spin levels due to quadrupolar splittings. Starting from known spin anisotropies we derive effective Hamiltonians in a generalized rotating frame, valid for arbitrary I, which allow us to describe the non-perturbative time evolution of spin states generated by magnetic rf fields. We identify an experimentally accessible regime where multiphoton Rabi oscillations are observable. In the nonlinear regime, we find Berry phase interference effects.

We consider an s-wave superconductor (SC) which is tunnel-coupled to two spatially separated Luttinger liquid (LL) leads. We demonstrate that such a setup acts as an entangler, i.e. it creates spin-singlets of two electrons which are spatially separated, thereby providing a source of electronic Einstein-Podolsky-Rosen pairs. We show that in the presence of a bias voltage, which is smaller than the energy gap in the SC, a stationary current of spin-entangled electrons can flow from the SC to the LL leads due to Andreev tunneling events. We discuss two competing transport channels for Cooper pairs to tunnel from the SC into the LL leads. On the one hand, the coherent tunneling of two electrons into the same LL lead is shown to be suppressed by strong LL correlations compared to single-electron tunneling into a LL. On the other hand, the tunneling of two spin-entangled electrons into different leads is suppressed by the initial spatial separation of the two electrons coming from the same Cooper pair. We show that the latter suppression depends crucially on the effective dimensionality of the SC. We identify a regime of experimental interest in which the separation of two spin-entangled electrons is favored. We determine the decay of the singlet state of two electrons injected into different leads caused by the LL correlations. Although the electron is not a proper quasiparticle of the LL, the spin information can still be transported via the spin density fluctuations produced by the injected spin-entangled electrons.

We study the decoherence of a single electron spin in an isolated quantum dot induced by hyperfine interaction with nuclei for times smaller than the nuclear spin relaxation time. The decay is caused by the spatial variation of the electron envelope wave function within the dot, leading to a non-uniform hyperfine coupling.
We evaluate the spin correlation function with and without magnetic fields and find that the decay of the spin precession amplitude is not exponential but rather power (inverse logarithm) law-like. For fully polarized nuclei we find an exact solution and show that the precession amplitude and the decay behavior can be tuned by the magnetic field.
The corresponding decay time is given by $\hbar N/A$, where $A$ is a hyperfine interaction constant and $N$ the number of nuclei inside the dot. The amplitude of precession, reached as a result of the decay, is finite. We show that there is a striking difference between the decoherence time for a single dot and the dephasing time for an ensemble of dots.

We discuss several scenarios for the creation of nonlocal spin-entangled electrons which provide a source of electronic Einstein-Podolsky-Rosen (EPR) pairs. Such EPR pairs can be used to test nonlocality of electrons in solid state systems, and they form the basic resources for quantum information processing. The central idea is to exploit the spin correlations naturally present in superconductors in form of Cooper pairs possessing spin-singlet wavefunctions. We show that nonlocal spin-entanglement in form of an effective Heisenberg spin interaction is induced between electron spins residing on two quantum dots with no direct coupling between them, but each of them being tunnel-coupled to the same superconductor. We then discuss a nonequilibrium setup with an applied bias where mobile and nonlocal spin-entanglement can be created by coherent injection of two electrons, in a pair (Andreev) tunneling process, into two spatially separated quantum dots and subsequently into two Fermi liquid leads. The current for injecting two spin-entangled electrons into different leads shows a resonance and allows the injection of electrons at the same orbital energy, which is a crucial requirement for the detection of spin-entanglement via the current noise. On the other hand, tunneling via the same dot into the same lead is suppressed by the Coulomb blockade effect of the quantum dots. We discuss Aharonov-Bohm oscillations in the current and show that they contain h/e and h/2e periods, which provides an experimental means to test the nonlocality of the entangled pair. Finally, we discuss a structure consisting of a superconductor weakly coupled to two separate one-dimensional leads with Luttinger liquid properties. We show that strong correlations again suppress the coherent subsequent tunneling of two electrons into the same lead, thus generating again nonlocal spin-entangled electrons in the Luttinger liquid leads.

Achieving control over the electron spin in quantum dots (artificial atoms) or real atoms promises access to new technologies in conventional and in quantum information processing. Here we review our proposal for quantum computing with spins of electrons confined to quantum dots. We discuss the basic requirements for implementing spin-qubits, and describe a complete set of quantum gates for single- and two-qubit operations. We show how a quantum dot attached to leads can be used for spin filtering and spin read-out, and as a spin-memory device. Finally, we focus on the experimental characterization of the quantum dot systems, and discuss transport properties of a double-dot and show how Kondo correlations can be used to measure the Heisenberg exchange interaction between the spins of two dots.

We give an elementary introduction to the notion of quantum entanglement between distinguishable parties and review a recent proposal about solid state quantum computation with spin-qubits in quantum dots. The indistinguishable character of the electrons whose spins realize the qubits gives rise to further entanglement-like quantum correlations. We summarize recent results concerning this type of quantum correlations of indistinguishable particles.

We investigate the spin dynamics of a quantum dot with a spin-1/2 ground state in the Coulomb blockade regime and in the presence of a magnetic rf field leading to electron spin resonances (ESR). We show that by coupling the dot to leads, spin properties on the dot can be accessed via the charge current in the stationary and non-stationary limit. We present a microscopic derivation of the current and the master equation of the dot using superoperators, including contributions to decoherence and energy shifts due to the tunnel coupling. We give a detailed analysis of sequential and co-tunneling currents, for linearly and circularly oscillating ESR fields, applied in cw and pulsed mode. We show that the sequential tunneling current exhibits a spin satellite peak whose linewidth gives a lower bound on the decoherence time T_2 of the dot-spin. Similarly, the spin decoherence can be accessed also in the cotunneling regime via ESR induced spin flips. We show that the conductance ratio of the spin satellite peak and the conventional peak due to sequential tunneling saturates at the universal conductance ratio of 0.71 for strong ESR fields. We describe a double-dot setup which generates spin dependent tunneling and acts as a current pump (at zero bias), and as a spin inverter which inverts the spin-polarization of the current. We show that Rabi oscillations of the dot-spin induce coherent oscillations in the time-dependent current. These oscillations are observable in the time-averaged current as function of ESR pulse-duration, and they allow one to access the spin coherence directly in the time domain. We analyze the measurement and read-out process of the dot-spin via currents in spin-polarized leads and identify measurement time and efficiency by calculating the counting statistics, noise, and the Fano factor.

We study biexcitonic states in two tunnel-coupled semiconductor quantum dots and show that they provide a source for entangled photons which are spatially separated at production. We distinguish between the various spin configurations and calculate the low-energy biexciton spectrum using the Heitler-London approximation as a function of magnetic and electric fields. We calculate the oscillator strengths for the biexciton recombination involving the sequential emission of two photons with entangled polarizations corresponding to the spin configuration in the biexciton states.

We present detailed calculations of low-energy spin dynamics in the ``ferric wheel'' systems Na:Fe_6 and Cs:Fe_8 in a magnetic field. We compute by exact diagonalization the low-energy spectra and matrix elements for total-spin and N'eel-vector components, and thus the time-dependent correlation functions of these operators. We compare our results with semiclassical tunneling descriptions, and discuss their implications for mesoscopic quantum coherence, as well as for the experimental techniques to observe it, in molecular magnetic rings.

We study two tunnel-coupled quantum dots each with a spin 1/2 and attached to leads in the Coulomb blockade regime. We study the interplay between Kondo correlations and the singlet-triplet exchange splitting $K$ between the two spins. We calculate the cotunneling current with elastic and inelastic contributions and its renormalization due to Kondo correlations, away and at the degeneracy point K=0. We show that these Kondo correlations induce pronounced peaks in the conductance as function of magnetic field $B$, inter-dot coupling $t_0$, and temperature. Moreover, the long-range part of the Coulomb interaction becomes visibile due to Kondo correlations resulting in an additional peak in the conductance vs $t_0$ with a strong $B$-field dependence. These conductance peaks thus provide direct experimental access to $K$, and thus to a crucial control parameter for spin-based qubits and entanglement.

We study the effect of the spin-orbit interaction on quantum gate operations based on the spin exchange coupling where the qubit is represented by the electron spin in a quantum dot or a similar nanostructure. Our main result is the exact cancellation of the spin-orbit effects in the sequence producing the quantum XOR gate for the ideal case where the pulse shapes of the exchange and spin-orbit interactions are identical. For the non-ideal case, we show that the two pulse shapes can be made almost identical and that the gate error is strongly suppressed by two small parameters, the spin-orbit interaction constant and the smallness of the deviation of the two pulse shapes. Similarly, we show that the dipole-dipole interaction leads only to very small errors in the XOR gate.

We study theoretically the spin dynamics of the ferric wheel, an antiferromagnetic molecular ring. For a single nuclear or impurity spin coupled to one of the electron spins of the ring, we calculate nuclear and electronic spin correlation functions and show that nuclear magnetic resonance (NMR) and electron spin resonance (ESR) techniques can be used to detect coherent tunneling of the Neel vector in these rings. The location of the NMR/ESR resonances gives the tunnel splitting and its linewidth an upper bound on the decoherence rate of the electron spin dynamics. We illustrate the experimental feasibility of our proposal with estimates for Fe_10 molecules.

We study theoretically the thermodynamic properties and spin dynamics of a class of magnetic rings closely related to ferric wheels, antiferromagnetic ring systems, in which one of the Fe (III) ions has been replaced by a dopant ion to create an excess spin. Using a coherent-state spin path integral formalism, we derive an effective action for the system in the presence of a magnetic field. We calculate the functional dependence of the magnetization and tunnel splitting on the magnetic field and show that the parameters of the spin Hamiltonian can be inferred from the magnetization curve. We study the spin dynamics in these systems and show that quantum tunneling of the Neel vector also results in tunneling of the total magnetization. Hence, the spin correlation function shows a signature of Neel vector tunneling, and electron spin resonance (ESR) techniques or AC susceptibility measurements can be used to measure both the tunneling and the decoherence rate. We compare our results with exact diagonalization studies on small ring systems. Our results can be easily generalized to a wide class of nanomagnets, such as ferritin.

We characterize and classify quantum correlations in two-fermion systems having 2K single-particle states. For pure states we introduce the Slater decomposition and rank (in analogy to Schmidt decomposition and rank), i.e. we decompose the state into a combination of elementary Slater determinants formed by mutually orthogonal single-particle states. Mixed states can be characterized by their Slater number which is the minimal Slater rank required to generate them. For K=2 we give a necessary and sufficient condition for a state to have a Slater number of 1. We introduce a correlation measure for mixed states which can be evaluated analytically for K=2. For higher K, we provide a method of constructing and optimizing Slater number witnesses, i.e. operators that detect Slater number for some states.

We propose the implementation of Grover's algorithm with molecular magnets with spin s>>1 in a unary representation. Shor and Grover demonstrated that a quantum computer can outperform any classical computer in factoring numbers[1] and in searching a database[2] by exploiting the parallelism of quantum mechanics. Whereas Shor's algorithm requires both superposition and entanglement of a many-particle system[3], the superposition of single-particle quantum states is sufficient for Grover's algorithm[4]. Recently, the latter has been successfully implemented[5] using Rydberg atoms. Here we propose an implementation of Grover's algorithm that uses molecular magnets[6,7,8,9,10], which are solid-state systems with a large spin; their spin eigenstates make them natural candidates for single-particle systems. We show theoretically that molecular magnets can be used to build dense and efficient memory devices based on the Grover algorithm. In particular, one single crystal can serve as a storage unit of a dynamic random access memory device. Fast electron spin resonance pulses can be used to decode and read out stored numbers of up to 105, with access times as short as 10-10 seconds. We show that our proposal should be feasible using the molecular magnets Fe8 and Mn12.

We consider a quantum dot attached to leads in the Coulomb blockade regime which has a spin 1/2 ground state. We show that by applying an ESR field to the dot-spin the stationary current in the sequential tunneling regime exhibits a resonance whose line width is determined by the single-spin decoherence time T_2. The Rabi oscillations of the dot-spin are shown to induce coherent current oscillations from which T_2 can be deduced in the time domain. We describe a spin-inverter which can be used to pump current through a double-dot via spin flips generated by ESR.

The organometallic ring molecules Fe_6 and Fe_10 are leading examples of a class of nanoscopic molecular magnets, which have been of intense recent interest both for their intrinsic magnetic properties and as candidates for the observation of macroscopic quantum coherent phenomena. Torque magnetometry experiments have been performed to measure the magnetization in single crystals of both systems. We provide a detailed interpretation of these results, with a view to full characterization of the material parameters. We present both the most accurate numerical simulations performed to date for ring molecules, using Exact Diagonalization and Density Matrix Renormalization Group techniques, and a semiclassical description for purposes of comparison. The results permit quantitative analysis of the variation of critical fields with angle, of the nature and height of magnetization and torque steps, and of the width and rounding of the plateau regions in both quantities.

We study the noise of the cotunneling current through one or several tunnel-coupled quantum dots in the Coulomb blockade regime. The various regimes of weak and strong, elastic and inelastic cotunneling are analyzed for quantum-dot systems (QDS) with few-level, nearly-degenerate, and continuous electronic spectra. We find that in contrast to sequential tunneling where the noise is either Poissonian (due to uncorrelated tunneling events) or sub-Poissonian (suppressed by charge conservation on the QDS), the noise in inelastic cotunneling can be super-Poissonian due to switching between QDS states carrying currents of different strengths. In the case of weak cotunneling we prove a non-equilibrium fluctuation-dissipation theorem which leads to a universal expression for the noise-to-current ratio (Fano factor). In order to investigate strong cotunneling we develop a microscopic theory of cotunneling based on the density-operator formalism and using the projection operator technique. The master equation for the QDS and the expressions for current and noise in cotunneling in terms of the stationary state of the QDS are derived and applied to QDS with a nearly degenerate and continuous spectrum.

We propose and analyze a spin-entangler for electrons based on an s-wave superconductor coupled to two quantum dots each of which is tunnel-coupled to normal Fermi leads. We show that in the presence of a voltage bias and in the Coulomb blockade regime two correlated electrons provided by the Andreev process can coherently tunnel from the superconductor via different dots into different leads. The spin-singlet coming from the Cooper pair remains preserved in this process, and the setup provides a source of mobile and nonlocal spin-entangled electrons. The transport current is calculated and shown to be dominated by a two-particle Breit-Wigner resonance which allows the injection of two spin-entangled electrons into different leads at exactly the same orbital energy, which is a crucial requirement for the detection of spin entanglement via noise measurements. The coherent tunneling of both electrons into the same lead is suppressed by the on-site Coulomb repulsion and/or the superconducting gap, while the tunneling into different leads is suppressed through the initial separation of the tunneling electrons. In the regime of interest the particle-hole excitations of the leads are shown to be negligible. The Aharonov-Bohm oscillations in the current are shown to contain single- and two-electron periods with amplitudes that both vanish with increasing Coulomb repulsion albeit differently fast.

Quantum computing and quantum communication are remarkable examples of new information processing technologies that arise from the coherent manipulation of spins in nanostructures. We review our theoretical proposal for using electron spins in quantum-confined nanostructures as qubits. We present single- and two-qubit gate mechanisms in laterally as well as vertically coupled quantum dots and discuss the possibility to couple spins in quantum dots via exchange or superexchange. In addition, we propose a new stationary wave switch, which allows to perform quantum operations with quantum dots or spin-1/2 molecules placed on a 1D or 2D lattice.

Quantum gates that temporarily increase singlet-triplet splitting in order to swap electronic spins in coupled quantum dots, lead inevitably to a finite double-occupancy probability for both dots. By solving the time-dependent Schröodinger equation for a coupled dot model, we demonstrate that this does not necessarily lead to quantum computation errors. Instead, the coupled dot ground state evolves quasi-adiabatically for typical system parameters so that the double-occupancy probability at the completion of swapping is negligibly small. We introduce a measure of entanglement which explicitly takes into account the possibilty of double occupancies and provides a necessary and sufficient criterion for entangled states.

We consider a quantum dot in the Coulomb blockade regime weakly coupled to current leads and show that in the presence of a magnetic field the dot acts as an efficient spin-filter (at the single-spin level) which produces a spin-polarized current. Conversely, if the leads are fully spin-polarized the up or down state of the spin on the dot results in a large sequential or small cotunneling current, and thus, together with ESR techniques, the setup can be operated as a single-spin memory.

The creation, coherent manipulation, and measurement of spins in nanostructures open up completely new possibilities for electronics and information processing, among them quantum computing and quantum communication. We review our theoretical proposal for using electron spins in quantum dots as quantum bits. We present single- and two qubit gate mechanisms in laterally as well as vertically coupled quantum dots and discuss the possibility to couple spins in quantum dots via superexchange. We further present the recently proposed schemes for using a single quantum dot as spin-filter and spin read-out/memory device. 

We present new topological interference effects for the tunneling of a single large spin, which are caused by the symmetry of a general class of magnetic anisotropies. The interference results from spin Berry phases associated with different tunneling paths exposed to the same dynamics. Introducing a generalized path integral for coherent spin states we evaluate transition amplitudes between ground as well as low-lying excited states. We show that these interference effects lead to topological selection rules and spin parity effects for integer spins which agree with quantum selection rules and which thus provide a generalization of the Kramers degeneracy to integer spins.

We use chiral Luttinger liquid theory to study transport through a quantum dot in the fractional quantum Hall effect regime and find rich non-Fermi-liquid tunneling characteristics. In particular, we predict a remarkable Coulomb-blockade-type energy gap that is quantized in units of the noninteracting level spacing, new power-law tunneling exponents for voltages beyond threshold, and a line shape as a function of gate voltage that is dramatically different than that for a Fermi liquid. We propose experiments to use these unique spectral properties as a new probe of the fractional quantum Hall effect.

We study a double quantum dot each dot of which is tunnel-coupled to superconducting leads. In the Coulomb blockade regime, a spin-dependent Josephson coupling between two superconductors is induced, as well as an antiferromagnetic Heisenberg exchange coupling between the spins on the double dot which can be tuned by the superconducting phase difference. We show that the correlated spin states-singlet or triplets-on the double dot can be probed via the Josephson current in a dc-SQUID setup.

Control over electron-spin states, such as coherent manipulation, filtering and measurement promises access to new technologies in conventional as well as in quantum computation and quantum communication. We review our proposal of using electron spins in quantum confined structures as qubits and discuss the requirements for implementing a quantum computer. We describe several realizations of one- and two-qubit gates and of the read-in and read-out tasks. We discuss recently proposed schemes for using a single quantum dot as spin-filter and spin-memory device. Considering electronic EPR pairs needed for quantum communication we show that their spin entanglement can be detected in mesoscopic transport measurements using metallic as well as superconducting leads attached to the dots.

We study Berry phase effects on conductance properties of diffusive mesoscopic conductors, which are caused by an electron spin moving through an orientationally inhomogeneous magnetic field. Extending previous work, we start with an exact, i.e. not assuming adiabaticity, calculation of the universal conductance fluctuations in a diffusive ring within the weak localization regime, based on a differential equation which we derive for the diffuson in the presence of Zeeman coupling to a magnetic field texture. We calculate the field strength required for adiabaticity and show that this strength is reduced by the diffusive motion. We demonstrate that not only the phases but also the amplitudes of the h/2e Aharonov-Bohm oscillations are strongly affected by the Berry phase. In particular, we show that these amplitudes are completely suppressed at certain magic tilt angles of the external fields, and thereby provide a useful criterion for experimental searches. We also discuss Berry phase-like effects resulting from spin-orbit interaction in diffusive conductors and derive exact formulas for both magnetoconductance and conductance fluctuations. We discuss the power spectra of the magnetoconductance and the conductance fluctuations for inhomogeneous magnetic fields and for spin-orbit interaction.

If the states of spins in solids can be created, manipulated, and measured at the single-quantum level, an entirely new form of information processing, quantum computing, will be possible.  We first give an overview of quantum information processing, showing that the famous Shor speedup of integer factoring is just one of a host of important applications for qubits, including cryptography, counterfeit protection, channel capacity enhancement, distributed computing, and others.  We review our proposed spin-quantum dot architecture for a quantum computer, and we indicate a variety of first generation materials, optical, and electrical measurements which should be considered. We analyze the efficiency of a two-dot device as a transmitter of quantum information via the  propagation of qubit carriers (i.e. electrons) in a Fermi sea. 

We consider a scattering set-up with an entangler and beam splitter where the current noise exhibits bunching behavior for electronic singlet states and antibunching behavior for triplet states. We show that the entanglement of two electrons in the double-dot can be detected in mesoscopic transport measurements. In the cotunneling regime the singlet and triplet states lead to phase-coherent current contributions of opposite signs and to Aharonov-Bohm and Berry phase oscillations in response to magnetic fields. We analyze the Fermi liquid effects in the transport of entangled electrons.

The creation, coherent manipulation, and measurement of spins in nanostructures open up completely new possibilities for electronics and information processing, among them quantum computing and quantum communication. We review our theoretical proposal for using electron spins in quantum dots as quantum bits, explaining why this scheme satisfies all the essential requirements for quantum computing. We include a discussion of the recent measurements of surprisingly long spin coherence times in semiconductors. Quantum gate mechanisms in laterally and vertically tunnel-coupled quantum dots and methods for single-spin measurements are introduced. We discuss detection and transport of electronic EPR pairs in normal and superconducting systems.

We determine the spin exchange coupling J between two electrons located in two vertically tunnel-coupled quantum dots, and its variation when magnetic (B) and electric (E) fields (both in-plane and perpendicular) are applied. We predict a strong decrease of J as the in-plane B field is increased, mainly due to orbital compression. Combined with the Zeeman splitting of the triplet, this leads to a singlet-triplet crossing, which can be observed as a pronounced jump in the magnetization, occurring at in-plane fields of a few Tesla, and perpendicular fields of the order of 10 Tesla for typical self-assembled dots. We use harmonic potentials to model the confining of electrons, and calculate the exchange J using the Heitler-London and Hund-Mulliken technique, including the long-range Coulomb interaction. With our results we provide experimental criteria for the distinction of singlet and triplet states and therefore for a microscopic spin measurement. In the case where quantum dots of different size are coupled, we present a simple method to switch on and off the spin coupling with exponential sensitivity using an in-plane electric field. Switching the spin coupling is essential for quantum computation using electronic spins as qubits.

Addressing the feasibilty of quantum communication with electrons we consider entangled spin states of electrons in a double-dot which is weakly coupled to in--and outgoing leads. We show that the entanglement of two electrons in the double-dot can be detected in mesoscopic transport and noise measurements. In the Coulomb blockade and cotunneling regime the singlet and triplet states lead to phase-coherent current and noise contributions of opposite signs and to Aharonov-Bohm and Berry phase oscillations in response to magnetic fields. These oscillations are a genuine two-particle effect and provide a direct measure of non-locality in entangled states. We show that the ratio of zero-frequency noise to current (Fano factor) is universal and equal to the electron charge.

In this chapter we explore the connection between mesoscopic physics and quantum computing.  After giving a bibliography providing a general introduction to the subject of quantum information processing, we review the various approaches that are being considered for the experimental implementation of quantum computing and quantum communication in atomic physics, quantum optics, nuclear magnetic resonance, superconductivity, and, especially, normal-electron solid state physics.  We discuss five criteria for the realization of a quantum computer and consider the implications that these criteria have for quantum computation using the spin states of single-electron quantum dots.  Finally, we consider the transport of quantum information via the motion of individual electrons in mesoscopic structures; specific transport and noise measurements in coupled quantum dot geometries for detecting and characterizing electron-state entanglement are analyzed.

We present a comprehensive theory of the magnetization relaxation in a Mn₁₂-acetate crystal in the high temperature regime (T>1K), which is based on phonon-assisted spin tunneling induced by quartic magnetic anisotropy and weak transverse magnetic fields. The overall relaxation rate as function of the longitudinal magnetic field is calculated and shown to agree well with experimental data including all resonance peaks measured so far. The Lorentzian shape of the resonances, which we obtain via a generalized master equation that includes spin tunneling, is also in good agreement with recent data. We derive a general formula for the tunnel splitting energy of these resonances. We show that fourth-order diagonal terms in the Hamiltonian lead to satellite peaks. A derivation of the effective linewidth of a resonance peak is given and shown to agree well with experimental data. In addition, previously unknown spin-phonon coupling constants are calculated explicitly. The values obtained for these constants and for the sound velocity are also in good agreement with recent data. We show that the spin relaxation in Mn₁₂-acetate takes place via several transition paths of comparable weight. These transition paths are expressed in terms of intermediate relaxation times, which are calculated and which can be tested experimentally.

We present a theoretical analysis of the properties of low-dimensional quantum antiferromagnets in applied magnetic fields. In a nonlinear sigma model description, we use a spin stiffness analysis, a 1/N expansion, and a renormalization group approach to describe the broken-symmetry regimes of finite magnetization, and, in cases of most interest, a low-field regime where symmetry is restored by quantum fluctuations. We compute the magnetization, critical fields, spin correlation functions, and decay exponents accessible by nuclear magnetic resonance experiments. The model is relevant to many systems exhibiting Haldane physics, and provides good agreement with data for the two-chain spin ladder compound CuHpCl. 

Addressing the feasibility of quantum communication with entangled electrons in an interacting many-body environment, we propose an interference experiment using a scattering set-up with an entangler and a beam splitter. It is shown that, due to electron-electron interaction, the delity of the entangled singlet and triplet states is reduced by z_F^2 in a conductor described by Fermi liquid theory. We calculate the quasiparticle weight factor z_F for a two-dimensional electron system. The current noise for electronic singlet states turns out to be enhanced (bunching behavior), while it is reduced for triplet states (antibunching). Within standard scattering theory, we nd that the Fano factor (noise-to-current ratio) for singlets is twice as large as for independent classical particles and is reduced to zero for triplets.

Pseudospin solitons in double-layer quantum Hall systems can be introduced by a magnetic field component coplanar with the electrons and can be pinned by applying voltages to external gates. We estimate the temperature below which depinning occurs predominantly via tunneling and calculate low-temperature depinning rates for realistic geometries.  We discuss the local changes in charge and current densities and in spectral functions that can be used to detect solitons and observe their temporal evolution. 

We generalize the Landau-Zener theory of coherent tunneling transitions by taking thermal relaxation into account. The evaluation of a new generalized master equation containing a dynamic tunneling rate that includes the interaction between the relevant system and its environment leads to an incoherent Zener transition probability with an exponent that is twice as large as the one of the coherent Zener probability in the limit T->0. We apply our results to molecular clusters, in particular to recent measurements of the tunneling transition of spins in Fe₈ crystals performed by Wernsdorfer and Sessoli  [Science 284, 133 (1999)].

We investigate Berry phase effects in the magnetoconductance of diffusive systems and determine the precise criterion for adiabaticity within the weak localization formalism. We show that  the exact solution of the Cooperon propagator for the special case of a cylindrically symmetric texture agrees with the adiabatic approximation in the adiabatic limit characterized by $\tau \gg {1\over d} {l²\over L²}$.  We point out that orientational inhomogeneities in the magnetic field induce dephasing effects that can mask the Berry phase (and any other phase coherent phenomena) for certain parameter values of system and field. 

Temperature-dependent magnetization measurements on a series of synthetic ferritin proteins containing from 100 to 3000 Fe(III) ions are used to determine the uncompensated moment of these antiferromagnetic particles. The results are compared with recent theories of macroscopic quantum coherence which explicitly include the effect of this excess moment. The scaling of the excess moment with protein size is consistent with a simple model of finite size effects and sublattice noncompensation. 

Quantum error correcting codes have been developed to protect a quantum computer from decoherence due to a noisy environment. In this paper, we present two methods for optimizing the physical implementation of such error correction schemes. First, we discuss an optimal quantum circuit implementation of the smallest error-correcting code (the three bit code). Quantum circuits are physically implemented by serial pulses, i.e. by switching on and off external parameters in the Hamiltonian one after another. In contrast to this, we introduce a new parallel switching method which allows faster gate operation by switching all external parameters simultaneously, and which has potential applications for arbitrary quantum computer architectures. We apply both serial and parallel switching to electron spins in coupled quantum dots subject to a Heisenberg coupling $H=J(t) S₁· S₂$. We provide a list of steps that can be implemented experimentally and used as a test for the functionality of quantum error correction. 

The electronic spin degrees of freedom in semiconductors typically have decoherence times that are several orders of magnitude longer than other relevant timescales. A solid-state quantum computer based on localized electron spins as qubits is therefore of potential interest. Here, a scheme that realizes controlled interactions between two distant quantum dot spins is proposed. The effective long-range interaction is mediated by the vacuum field of a high finesse microcavity. By using conduction-band-hole Raman transitions induced by classical laser fields and the cavity-mode, arbitrary single qubit rotations and controlled-not operations can be realized. Optical techniques can also be used to measure the spin-state of each quantum dot. 

We consider a new quantum gate mechanism based on electron spins in coupled semiconductor quantum dots.  Such gates provide a general source of spin entanglement and can be used for quantum computers.  We determine the exchange coupling $J$ in the effective Heisenberg model as a function of magnetic ($B$) and electric fields, and of the inter-dot distance $a$ within the Heitler-London approximation of molecular physics. This result is refined by using sp-hybridization, and by the Hund-Mulliken molecular-orbit approach which leads to an extended Hubbard description for the two-dot system that shows a remarkable dependence on $B$ and $a$ due to the long-range Coulomb interaction. We find that the exchange $J$ changes sign at a finite field (leading to a pronounced jump in the magnetization) and then decays exponentially.  The magnetization and the spin susceptibilities of the coupled dots are calculated.  We show that the dephasing due to nuclear spins in GaAs can be strongly suppressed by dynamical nuclear spin polarization and/or by magnetic fields. 

We study noise and transport in multiterminal diffusive conductors. Using a Boltzmann-Langevin equation approach we reduce the calculation of shot-noise correlators to the solution of diffusion equations. Within this approach we prove the universality of shot noise in multiterminal diffusive conductors of arbitrary shape and dimension for purely elastic scattering as well as for hot electrons. We show that shot noise in multiterminal conductors is a non-local quantity and that exchange effects can occur in the absence of quantum phase coherence even at zero electron temperature. It is also shown that the exchange effect measured in one contact is always negative -- in agreement with the Pauli principle. We discuss a new phenomenon in which current noise is induced by thermal transport. We propose a possible experiment to measure locally the effective noise temperature. Concrete numbers for shot noise are given that can be tested experimentally. 

We propose a new implementation of a universal set of one- and two-qubit gates for quantum computation using the spin states of coupled single-electron quantum dots.  Desired operations are effected by the gating of the tunneling barrier between neighboring dots. Several measures of the gate quality are computed within a newly derived spin master equation incorporating decoherence caused by a prototypical magnetic environment.  Dot-array experiments which would provide an initial demonstration of the desired non-equilibrium spin dynamics are proposed. 

A review of quantum coherence effects in mesoscopic  spin systems is presented. We  begin with a general introduction to the topic of mesoscopic effects in magnetism and give some specific examples of current interest. We review then theoretical results in single domain magnetism of superparamagnetic type and mention  recent measurements on antiferromagnetic  grains (ferritin) and their interpretation in terms of macroscopic quantum coherence. Introducing the effects originating from  spin parity in the context of ferromagnetic grains, we discuss antiferromagnetic particles with excess spins and  molecular magnets such as the ferric wheel. It is shown that tunneling in such magnets can be tuned by external magnetic fields and is directly observable via the magnetization and the Schottky anomaly in the specific heat. The main part of the review  will be devoted to non-uniform magnets and specifically to the   quantum dynamics of domain walls or magnetic solitons.  In a semiclassical analysis based on coherent spin-state path-integrals an effective model for the  domain wall dynamics is derived which includes the effects of spin-wave dissipation and of quantum spin phases (Berry phases). In the presence of a Peierls potential (e.g. due to the discrete lattice)  the soliton center can tunnel coherently between the lattice sites and form a Bloch band. Integer and half-odd integer spins have different energy dispersions resulting from interference between soliton states of opposite chirality--the internal rotation sense of the soliton. These effects occur in ferro- and antiferromagnets due to the presence of a topological spin phase. For antiferromagnetic chains, this spin phase occurs in addition to the Pontryagin-index phase.We will discuss  experimental consequences of this Bloch band structure and  show that ---in analogy to Bloch oscillations of crystal electrons--- static magnetic fields induce large oscillations in the sample magnetization. We will also discuss the extreme quantum limit of spin-1/2 chains in the Ising regime, and show that, quite remarkably, the semiclassical analysis  is valid even in this regime. In particular, for antiferromagnetic Ising chains the low-energy excitations are solitons (Villain modes) which have  been observed in neutron scattering experiments on CsCoCl₃. We show that the prediction of chirality effects could be tested via the measurement of the off-diagonal components of the dynamical structure factor. The concept of chirality is shown to be of universal character in a variety of magnetic systems, a notable example being the motion of a hole in a 2D antiferromagnetic background. A common thread in the discussion of quantum dynamics in magnets is provided by the Berry phases and their associated interference effects which can lead to surprising spin parity effects. 

We study macroscopic quantum coherence in antiferromagnetic molecular magnets in the presence of magnetic fields. Such fields generate artificial tunnel barriers with externally tunable strength.  We give detailed semi-classical predictions for the tunnel splitting in various regimes for low and high magnetic fields. We show that the tunneling dynamics of the N\'eel vector can be directly measured via the static magnetization and the specific heat.  We also report on a new quantum phase arising from fluctuations. The analytic results are complemented by numerical simulations. 

We study the quantum dynamics of soliton-like domain walls in anisotropic spin-1/2 chains in the presence of magnetic fields. In the absence of fields, domain walls form a Bloch band of delocalized quantum states while a static field applied along the easy axis localizes them into Wannier wave packets and causes them to execute Bloch oscillations, i.e.\ the domain walls oscillate along the chain with a finite Bloch frequency and amplitude.  In the presence of the field, the Bloch band, with a continuum of extended states, breaks up into the Wannier-Zeeman ladder---a discrete set of equally spaced energy levels.  We calculate the dynamical structure factor $S^zz (q,\omega)$ in the one-soliton sector at finite frequency, wave vector, and temperature, and find sharp peaks at frequencies which are integer multiples of the Bloch frequency.  We further calculate the uniform magnetic susceptibility and find that it too exhibits peaks at the Bloch frequency.  We identify several candidate materials where these Bloch oscillations should be observable, for example, via neutron scattering measurements. For the particular compound ${\rm CoCl₂ \!  · \!  2H₂O}$ we estimate the Bloch amplitude to be on the order of a few lattice constants, and the Bloch frequency on the order of 100\,GHz for magnetic fields in the Tesla range and at temperatures of about 18\,Kelvin. 

We study macroscopic quantum coherence (MQC) in small magnetic particles where the magnetization (in ferromagnets) or the N\'eel vector (in antiferromagnets) can tunnel between energy minima.  We consider here the more general case of MQC in ferrimagnets by studying a model for a mesoscopic antiferromagnet with an uncompensated magnetic moment.  Through semi-classical calculations we show that even a small moment has a drastic effect on MQC. In particular, there is a rapid crossover to a regime where the MQC tunnel splitting is equal to that obtained for a ferromagnet, even though the system is still an antiferromagnet for all other aspects.  We calculate this tunnel splitting via instanton methods and compare it with numerical evaluations. As an application we re-examine the experimental evidence for MQC in ferritin and show that even though the  uncompensated  moment of ferritin is small it greatly modifies the MQC behavior. The excess spin allows us to extract values for experimental parameters without making any assumption about the classical attempt frequency, in contrast to previous fits. Finally, we also discuss the implications of our results for MQC in molecular magnets. 

Edge states of the quantum Hall fluid provide an almost unparalled opportunity to study mesoscopic effects in a highly correlated electron system. In this paper we develop a bosonization formalism for the finite-size edge state, as described by chiral Luttinger liquid theory, and use it to study the Aharonov-Bohm effect. We study tunneling through an edge state formed around an antidot in the fractional quantum Hall regime using Wen's chiral Luttinger liquid theory extended to include mesoscopic effects. We identify a new regime where the Aharonov-Bohm oscillation amplitude exhibits a distinctive crossover from Luttinger liquid power-law behavior to Fermi-liquid-like behavior as the temperature is increased. Near the crossover temperature the amplitude has a pronounced maximum. This non-monotonic behavior and  novel high-temperature nonlinear phenomena that we also predict provide new ways to distinguish experimentally between Luttinger and Fermi liquids. Finally, we predict new mesoscopic edge-current oscillations, which are similar to the persistent currentoscillations in a mesoscopic ring, except that they are not reduced in amplitude by weak disorder. In the fractional quantum Hall regime, these ``chiral persistent currents'' have a universal non-Fermi-liquid temperature dependence and may be another ideal system to observe a chiral Luttinger liquid. 

Quantum tunneling of domain walls out of an impurity potential in a mesoscopic ferromagnetic sample is investigated.  Using improved expressions for the domain wall mass and for the pinning potential, we find that the cross-over temperature between thermal activation and quantum tunneling is of a different functional form than found previously. In materials like Ni or YIG, the crossover temperatures are around 5 mK. We also find that the WKB exponent is typically two orders of magnitude larger than current estimates. The sources for these discrepancies are discussed, and precise estimates for the transition from three-dimensional to one-dimensional magnetic behavior of a wire are given. The cross-over temperatures from thermal to quantum transitions and tunneling rates are calculated for various materials and sample sizes.

We study tunneling through an edge state formed around an antidot in the fractional quantum Hall regime using Wen's chiral Luttinger liquid theory extended to include mesoscopic effects. We identify a new regime where the Aharonov-Bohm oscillation amplitude exhibits a distinctive crossover from Luttinger liquid power-law behavior to Fermi-liquid-like behavior as the temperature is increased. Near the crossover temperature the amplitude has a pronounced maximum. This non-monotonic behavior and novel high-temperature nonlinear phenomena that we also predict provide new ways to distinguish experimentally between Luttinger and Fermi liquids.

We study spin parity effects and the quantum propagation of solitons "Bloch walls" in quasi-one-dimensional ferromagnets. Within a coherent state path integral approach we derive a quantum field theory for nonuniform spin configurations. The effective action for the soliton position is shown to contain a gauge potential due to the Berry phase and a damping term caused by the interaction between soliton and spin waves. For tempera- tures below the anisotropy gap this dissipation reduces to a pure soliton mass renormalization. The quantum dynamics of the soliton in a periodic lattice or pinning potential reveals remarkable consequences of the Berry phase. For half-integer spin, destructive interference between opposite chiralities suppresses nearest-neighbor hopping. Thus the Brillouin zone is halved, and for small mixing of the chiralities the dispersion reveals a surprising dynamical correlation: Two subsequent band minima belong to different chirality states of the soliton. For integer spin the Berry phase is inoperative and a simple tight-binding dispersion is obtained. Finally it is shown that external fields can be used to interpolate continuously between the Bloch wall disper- sions for half-integer and integer spin.